Department of Applied Physics, Chalmers University of Technology, Goteborg, Sweden.
Nano Lett. 2010 Jan;10(1):268-73. doi: 10.1021/nl9034434.
We demonstrate optical alignment and rotation of individual plasmonic nanostructures with lengths from tens of nanometers to several micrometers using a single beam of linearly polarized near-infrared laser light. Silver nanorods and dimers of gold nanoparticles align parallel to the laser polarization because of the high long-axis dipole polarizability. Silver nanowires, in contrast, spontaneously turn perpendicular to the incident polarization and predominantly attach at the wire ends, in agreement with electrodynamics simulations. Wires, rods, and dimers all rotate if the incident polarization is turned. In the case of nanowires, we demonstrate spinning at an angular frequency of approximately 1 Hz due to transfer of spin angular momentum from circularly polarized light.
我们使用一束线偏振的近红外激光演示了长度从几十纳米到几微米的单个等离子体纳米结构的光学对准和旋转。由于长轴偶极极化率高,银纳米棒和金纳米粒子的二聚体与激光偏振平行排列。相比之下,银纳米线会自发地垂直于入射偏振方向,并主要附着在线的末端,这与电动力学模拟结果一致。如果入射偏振发生变化,纳米线、纳米棒和二聚体都会发生旋转。在纳米线的情况下,我们证明了由于圆偏振光的自旋角动量转移,纳米线以大约 1 Hz 的角频率旋转。