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悬浮于硬球样粒子中的粒子电流的时空关联函数的标度:揭示粒子运动为布朗运动时的情况。

Scaling of the space-time correlation function of particle currents in a suspension of hard-sphere-like particles: exposing when the motion of particles is Brownian.

机构信息

Department of Applied Physics, Royal Melbourne Institute of Technology, Melbourne, Victoria 3000, Australia.

出版信息

Phys Rev Lett. 2009 Dec 18;103(25):258302. doi: 10.1103/PhysRevLett.103.258302. Epub 2009 Dec 17.

Abstract

The current correlation function is determined from dynamic light scattering measurements of a suspension of particles with hard spherelike interactions. For suspensions in thermodynamic equilibrium we find scaling of the space and time variables of the current correlation function. This finding supports the notion that the movement of suspended particles can be described in terms of uncorrelated Brownian encounters. However, in the metastable fluid, at volume fractions above freezing, this scaling fails.

摘要

当前的相关函数是通过对具有硬球相互作用的粒子悬浮液的动态光散射测量来确定的。对于处于热力学平衡的悬浮液,我们发现电流相关函数的空间和时间变量的标度。这一发现支持了这样一种观点,即悬浮颗粒的运动可以用无关联的布朗遭遇来描述。然而,在亚稳流体中,在过冷的体积分数以上,这种标度失效了。

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