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支撑石墨烯中的二维声子输运。

Two-dimensional phonon transport in supported graphene.

机构信息

Department of Mechanical Engineering, The University of Texas at Austin, Austin, TX 78712, USA.

出版信息

Science. 2010 Apr 9;328(5975):213-6. doi: 10.1126/science.1184014.

Abstract

The reported thermal conductivity (kappa) of suspended graphene, 3000 to 5000 watts per meter per kelvin, exceeds that of diamond and graphite. Thus, graphene can be useful in solving heat dissipation problems such as those in nanoelectronics. However, contact with a substrate could affect the thermal transport properties of graphene. Here, we show experimentally that kappa of monolayer graphene exfoliated on a silicon dioxide support is still as high as about 600 watts per meter per kelvin near room temperature, exceeding those of metals such as copper. It is lower than that of suspended graphene because of phonons leaking across the graphene-support interface and strong interface-scattering of flexural modes, which make a large contribution to kappa in suspended graphene according to a theoretical calculation.

摘要

所报道的悬浮石墨烯的热导率(kappa)为 3000 至 5000 瓦/米/开尔文,超过了金刚石和石墨。因此,石墨烯在解决纳米电子学中的散热问题等方面可能很有用。然而,与衬底接触可能会影响石墨烯的热输运性能。在这里,我们通过实验表明,在二氧化硅衬底上剥离的单层石墨烯在室温附近的热导率仍高达约 600 瓦/米/开尔文,超过了铜等金属的热导率。由于声子穿过石墨烯-衬底界面泄漏以及弯曲模式的强界面散射,其值低于悬浮石墨烯,根据理论计算,这些模式对悬浮石墨烯的 kappa 有很大贡献。

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