Center for Biomedical Engineering and Technology, University of Maryland, Baltimore, MD 21201, USA.
J Mol Biol. 2010 Jul 23;400(4):908-21. doi: 10.1016/j.jmb.2010.05.051. Epub 2010 May 27.
It has been well established that a single amino acid sequence can give rise to several conformationally distinct amyloid states. The extent to which amyloid structures formed within the same sequence are different, however, remains unclear. To address this question, we studied two amyloid states (referred to as R- and S-fibrils) produced in vitro from highly purified full-length recombinant prion protein. Several biophysical techniques including X-ray diffraction, CD, Fourier transform infrared spectroscopy (FTIR), hydrogen-deuterium exchange, proteinase K digestion, and binding of a conformation-sensitive fluorescence dye revealed that R- and S-fibrils have substantially different secondary, tertiary, and quaternary structures. While both states displayed a 4. 8-A meridional X-ray diffraction typical for amyloid cross-beta-spines, they showed markedly different equatorial profiles, suggesting different folding pattern of beta-strands. The experiments on hydrogen-deuterium exchange monitored by FTIR revealed that only small fractions of amide protons were protected in R- or S-fibrils, an argument for the dynamic nature of their cross-beta-structure. Despite this fact, both amyloid states were found to be very stable conformationally as judged from temperature-induced denaturation monitored by FTIR and the conformation-sensitive dye. Upon heating to 80 degrees C, only local unfolding was revealed, while individual state-specific cross-beta features were preserved. The current studies demonstrated that the two amyloid states formed by the same amino acid sequence exhibited significantly different folding patterns that presumably reflect two different architectures of cross-beta-structure. Both S- and R-fibrils, however, shared high conformational stability, arguing that the energy landscape for protein folding and aggregation can contain several deep free-energy minima.
已经证实,单一的氨基酸序列可以产生几种构象上明显不同的淀粉样状态。然而,在同一序列中形成的淀粉样结构在多大程度上有所不同尚不清楚。为了解决这个问题,我们研究了两种体外产生的高度纯化全长重组朊病毒蛋白的淀粉样状态(称为 R-和 S-原纤维)。几种生物物理技术,包括 X 射线衍射、CD、傅里叶变换红外光谱(FTIR)、氢氘交换、蛋白酶 K 消化以及构象敏感荧光染料的结合,表明 R-和 S-原纤维具有显著不同的二级、三级和四级结构。虽然两种状态都显示出典型的 4.8-A 子午线 X 射线衍射,表明淀粉样交叉-β-棘突,但它们表现出明显不同的赤道轮廓,表明β-折叠的折叠模式不同。FTIR 监测的氢氘交换实验表明,R-或 S-原纤维中只有少量酰胺质子被保护,这表明其交叉-β-结构具有动态性质。尽管如此,根据 FTIR 监测的温度诱导变性和构象敏感染料,两种淀粉样状态都被发现具有非常稳定的构象。在 80°C 加热时,仅揭示了局部展开,而保留了各个状态特异性的交叉-β 特征。目前的研究表明,由相同氨基酸序列形成的两种淀粉样状态表现出明显不同的折叠模式,这可能反映了交叉-β-结构的两种不同架构。然而,S-和 R-原纤维都具有很高的构象稳定性,这表明蛋白质折叠和聚集的能量景观可以包含几个深的自由能最小值。