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利用纳米等离子体学控制光局域和光物质相互作用。

Controlling light localization and light-matter interactions with nanoplasmonics.

机构信息

Department of Physics, Imperial College London, London SW7 2AZ, United Kingdom.

出版信息

Small. 2010 Nov 22;6(22):2498-507. doi: 10.1002/smll.201001044.

Abstract

Nanoplasmonics is the emerging research field that studies light-matter interactions mediated by resonant excitations of surface plasmons in metallic nanostructures. It allows the manipulation of the flow of light and its interaction with matter at the nanoscale (10(-9) m). One of the most promising characteristics of plasmonic resonances is that they occur at frequencies corresponding to typical electronic excitations in matter. This leads to the appearance of strong interactions between localized surface plasmons and light emitters (such as molecules, dyes, or quantum dots) placed in the vicinity of metals. Recent advances in nanofabrication and the development of novel concepts in theoretical nanophotonics have opened the way to the design of structures aimed to reduce the lifetime and enhance the decay rate and quantum efficiency of available emitters. In this article, some of the most relevant experimental and theoretical achievements accomplished over the last several years are presented and analyzed.

摘要

纳米等离子体学是一个新兴的研究领域,研究由金属纳米结构中表面等离激元的共振激发介导的光物质相互作用。它允许在纳米尺度(10^-9 米)上操纵光的流动及其与物质的相互作用。等离子体共振的最有前途的特性之一是它们发生在与物质中典型的电子激发相对应的频率处。这导致了局部表面等离激元和放置在金属附近的光发射器(如分子、染料或量子点)之间的强相互作用的出现。纳米制造的最新进展和理论纳米光子学的新概念的发展为设计旨在减少寿命和提高现有发射器的衰减率和量子效率的结构开辟了道路。本文介绍并分析了过去几年中取得的一些最相关的实验和理论成果。

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