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采用扫描热显微镜和空间分辨拉曼光谱相结合的方法研究载流 GaN 纳米线中的定量散热特性。

Quantitative heat dissipation characteristics in current-carrying GaN nanowires probed by combining scanning thermal microscopy and spatially resolved Raman spectroscopy.

机构信息

Department of Physics and Astronomy, Washington State University, Pullman, Washington 99164, United States.

出版信息

ACS Nano. 2011 Jan 25;5(1):255-62. doi: 10.1021/nn102818s. Epub 2010 Dec 14.

DOI:10.1021/nn102818s
PMID:21155591
Abstract

Using an approach combining scanning thermal microscopy (SThM) and spatially revolved Raman spectroscopy, we have investigated quantitatively the heat dissipation characteristics in substrate-supported and suspended (with asymmetric type of contacts) current-carrying GaN nanowires with diameters of ∼40-60 nm, where the phonon confinement is expected to play an important role in thermal transport. In particular, this approach allows direct measurements of nanowire-substrate/electrode interface thermal resistances and the nanowire thermal conductivity. On the basis of these results, the nanowire-substrate thermal transfer was suggested to be the main heat dissipation route, counting for ∼80-93% of the total dissipated heat, whereas the nanowire-electrode interface plays a minor role. The relative significance of nanowire-substrate/electrode interfaces in dissipating heat was further demonstrated in suspended nanowire devices. The measured nanowire thermal conductivity (∼40-60 W/mK) is lower than that in bulk GaN, possibly due to the phonon confinement and boundary scattering effects. Besides providing quantitative insight into heat dissipation characteristics, our results also reveal aspects, particularly the topography-related thermal signals and the relative significance of various tip-sample thermal transfer processes, that are important to advancing the applications of SThM technique in nanoscale thermal characterizations.

摘要

我们采用扫描热显微镜(SThM)和空间旋转拉曼光谱相结合的方法,对直径约为 40-60nm 的衬底支撑和悬浮(具有不对称类型接触)电流承载 GaN 纳米线的散热特性进行了定量研究,其中声子限制在热输运中起着重要作用。特别是,这种方法允许直接测量纳米线-衬底/电极界面热阻和纳米线热导率。基于这些结果,纳米线-衬底热传递被认为是主要的散热途径,占总耗散热量的 80-93%,而纳米线-电极界面的作用较小。在悬浮纳米线器件中进一步证明了纳米线-衬底/电极界面在散热方面的相对重要性。测量的纳米线热导率(约 40-60W/mK)低于体 GaN 的热导率,这可能是由于声子限制和边界散射效应。除了提供对散热特性的定量见解外,我们的结果还揭示了一些方面,特别是与形貌相关的热信号和各种针尖-样品热传递过程的相对重要性,这对于推进 SThM 技术在纳米尺度热特性中的应用具有重要意义。

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