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单壁碳纳米管热电堆用于宽带光探测。

Single-walled carbon nanotube thermopile for broadband light detection.

机构信息

Regroupement Québécois sur les Matériaux de Pointe (RQMP), Montréal QC, Canada.

出版信息

Nano Lett. 2011 Feb 9;11(2):609-13. doi: 10.1021/nl1036947. Epub 2010 Dec 28.

Abstract

We designed a thermopile based on a PN doping profile engineered in a suspended film of single-walled carbon nanotubes (SWNTs). Using estimates of the film local Seebeck coefficients, the SWNT thermopile was optimized in situ through depositions of potassium dopants. The overall performances of the thermopile were found to be comparable to state-of-the-art SWNT bolometers. The device is characterized at room temperature by a time response of 36 ms, typical of thermal detectors, and an optimum spectral detectivity of 2 × 10(6) cm Hz(1/2)/W in the visible and near-infrared. This paper presents the first thermopile made of a suspended SWNT film and paves the way to new applications such as broadband light (including THz) detection and thermoelectric power generation.

摘要

我们设计了一种基于在悬浮的单壁碳纳米管(SWNTs)薄膜中进行的 PN 掺杂分布的热堆。利用对薄膜局部塞贝克系数的估计,通过钾掺杂剂的沉积,对 SWNT 热堆进行了原位优化。发现热堆的整体性能可与最先进的 SWNT 测辐射热计相媲美。该器件在室温下的时间响应为 36ms,与热探测器典型值相当,在可见光和近红外光范围内的最佳光谱探测率为 2×10(6)cmHz(1/2)/W。本文介绍了第一个由悬浮的 SWNT 薄膜制成的热堆,为新的应用铺平了道路,例如宽带光(包括太赫兹)检测和热电发电。

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