Advanced Study Program, National Center for Atmospheric Research, Boulder, CO 80307, USA.
Proc Natl Acad Sci U S A. 2011 Jan 18;108(3):1016-21. doi: 10.1073/pnas.1014798108. Epub 2010 Dec 28.
Mineral dust aerosols impact Earth's radiation budget through interactions with clouds, ecosystems, and radiation, which constitutes a substantial uncertainty in understanding past and predicting future climate changes. One of the causes of this large uncertainty is that the size distribution of emitted dust aerosols is poorly understood. The present study shows that regional and global circulation models (GCMs) overestimate the emitted fraction of clay aerosols (< 2 μm diameter) by a factor of ∼2-8 relative to measurements. This discrepancy is resolved by deriving a simple theoretical expression of the emitted dust size distribution that is in excellent agreement with measurements. This expression is based on the physics of the scale-invariant fragmentation of brittle materials, which is shown to be applicable to dust emission. Because clay aerosols produce a strong radiative cooling, the overestimation of the clay fraction causes GCMs to also overestimate the radiative cooling of a given quantity of emitted dust. On local and regional scales, this affects the magnitude and possibly the sign of the dust radiative forcing, with implications for numerical weather forecasting and regional climate predictions in dusty regions. On a global scale, the dust cycle in most GCMs is tuned to match radiative measurements, such that the overestimation of the radiative cooling of a given quantity of emitted dust has likely caused GCMs to underestimate the global dust emission rate. This implies that the deposition flux of dust and its fertilizing effects on ecosystems may be substantially larger than thought.
矿物质粉尘气溶胶通过与云、生态系统和辐射的相互作用影响地球的辐射平衡,这构成了理解过去和预测未来气候变化的一个重大不确定性。造成这种巨大不确定性的原因之一是,对排放粉尘气溶胶的大小分布了解甚少。本研究表明,区域和全球环流模型(GCM)对粘土气溶胶(<2μm 直径)的排放部分的估计值比测量值高约 2-8 倍。通过推导出与测量值非常吻合的简单粉尘排放大小分布的理论表达式,解决了这一差异。该表达式基于脆性材料的标度不变碎裂的物理原理,表明该原理适用于粉尘排放。由于粘土气溶胶产生强烈的辐射冷却,粘土部分的高估导致 GCM 也高估了给定数量的排放粉尘的辐射冷却。在局部和区域尺度上,这会影响尘埃辐射强迫的大小,甚至可能改变其符号,这对多尘地区的数值天气预报和区域气候预测有影响。在全球范围内,大多数 GCM 中的尘埃循环被调整以匹配辐射测量,因此,对给定数量的排放粉尘的辐射冷却的高估可能导致 GCM 低估了全球尘埃排放率。这意味着尘埃的沉积通量及其对生态系统的施肥效应可能比人们想象的要大得多。