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Xe@C₆₀+ 光电离中的禁闭共振。

Confinement resonances in photoionization of Xe@C₆₀+.

机构信息

Advanced Light Source, LBNL, MS 7-100, Berkeley, California 94720-8225, USA.

出版信息

Phys Rev Lett. 2010 Nov 19;105(21):213001. doi: 10.1103/PhysRevLett.105.213001. Epub 2010 Nov 15.

Abstract

Experimental evidence is presented for confinement resonances associated with photoabsorption by a Xe atom in a C60 cage. The giant 4d resonance in photoionization of Xe is predicted to be redistributed into four components due to multipath interference of photoelectron waves reflected by the cage. The measurements were made in the photon energy range 60-150 eV by merging a beam of synchrotron radiation with a mass/charge selected Xe@C₆₀+ ion beam. The phenomenon was observed in the Xe@C(58)(3+) product ion channel. [corrected]

摘要

实验证据表明,与 Xe 原子在 C60 笼中光吸收相关的限制共振。由于笼反射的光电子波的多路径干扰,预测 Xe 的光致电离中的巨大 4d 共振将重新分布为四个分量。在光子能量范围为 60-150 eV 时,通过将同步加速器辐射束与质量/电荷选择的 Xe@C₆₀+离子束合并来进行测量。该现象在 Xe@C(58)(3+)产物离子通道中被观察到。[已更正]

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