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量子点-金属纳米粒子分子的量子等离子体学:费诺效应对光子统计的影响。

Quantum plasmonics with quantum dot-metal nanoparticle molecules: influence of the Fano effect on photon statistics.

机构信息

Dipartimento di Fisica della Materia e Ingegneria Elettronica, Università di Messina, Messina, Italy.

出版信息

Phys Rev Lett. 2010 Dec 31;105(26):263601. doi: 10.1103/PhysRevLett.105.263601. Epub 2010 Dec 20.

Abstract

We study theoretically the quantum optical properties of hybrid molecules composed of an individual quantum dot and a metallic nanoparticle. We calculate the resonance fluorescence of this composite system. Its incoherent part, arising from nonlinear quantum processes, is enhanced by more than 2 orders of magnitude as compared to that of the dot alone. The coupling between the two systems gives rise to a Fano interference effect which strongly influences the quantum statistical properties of the scattered photons: a small frequency shift of the incident light field may cause changes in the intensity correlation function of the scattered field of orders of magnitude. The system opens a good perspective for applications in active metamaterials and ultracompact single-photon devices.

摘要

我们从理论上研究了由单个量子点和金属纳米粒子组成的混合分子的量子光学性质。我们计算了这个复合系统的共振荧光。与单独的点相比,其由非线性量子过程引起的非相干部分增强了两个数量级以上。两个系统之间的耦合产生了一种 Fano 干涉效应,强烈影响散射光子的量子统计性质:入射光场的小频率位移可能导致散射场强度相关函数发生数量级的变化。该系统为应用于有源超材料和超紧凑型单光子器件开辟了良好的前景。

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