Jacob F, Joris B, Dideberg O, Dusart J, Ghuysen J M, Frère J M
Laboratoire d'Enzymologie, Institut de Chimie, Université de Liège, Belgium.
Protein Eng. 1990 Oct;4(1):79-86. doi: 10.1093/protein/4.1.79.
beta-Lactamases are widespread and efficient bacterial enzymes which play a major role in bacterial resistance to penicillins and cephalosporins. In order to elucidate the role of the residues lying in a conserved loop of the enzymatic cavity of the active-site serine Streptomyces albus G beta-lactamase, modified proteins were produced by oligo-directed mutagenesis. Mutation of Asn116, which lies on one side of the active site cavity pointing to the substrate-binding site, into a serine residue resulted in spectacular modifications of the specificity profile of the enzyme. That replacement yielded an enzyme with a nearly unchanged activity towards good penicillin substrates. In sharp contrast its efficiency in hydrolysing cephalosporins was drastically reduced, the best substrates suffering the largest decrease in the second-order rate constant for serine acylation. In fact that single mutation generated a truly new enzyme behaving exclusively as a penicillinase, a situation which is never encountered to the same degree in any of the numerous naturally occurring variants of class A beta-lactamases.
β-内酰胺酶是广泛存在且高效的细菌酶,在细菌对青霉素和头孢菌素的耐药性中起主要作用。为了阐明位于活性位点丝氨酸链霉菌Gβ-内酰胺酶酶腔保守环中的残基的作用,通过寡核苷酸定向诱变产生了修饰蛋白。位于活性位点腔一侧指向底物结合位点的Asn116突变为丝氨酸残基,导致该酶的特异性谱发生显著改变。这种替换产生了一种对良好青霉素底物活性几乎不变的酶。与之形成鲜明对比的是,其水解头孢菌素的效率大幅降低,最佳底物的丝氨酸酰化二级速率常数下降幅度最大。事实上,单一突变产生了一种全新的酶,仅表现为青霉素酶,这种情况在A类β-内酰胺酶的众多天然变体中从未达到相同程度。