Department of Molecular Therapeutics, The Scripps Research Institute, Scripps Florida, Jupiter, FL 33458, United States.
ACS Chem Biol. 2011 Jun 17;6(6):618-27. doi: 10.1021/cb100396s. Epub 2011 Mar 17.
Retinoids are potent forms of vitamin A and are involved in a broad range of physiological processes and the pharmacological effects of retinoids are primarily mediated by the retinoic acid receptors (RARs) and the retinoid X receptors (RXRs). Several natural and synthetic RAR modulators have proven to be clinically useful for a number of therapeutic indications including cancer, psoriasis, and diabetes. Unfortunately, these agents lead to a number of significant side effects. Most synthetic retinoid ligands are based on the retinoid scaffold and thus have similarities to the natural ligand with all previously disclosed RAR ligands having a carboxylic acid that makes a critical ionic bridge within the ligand binding domain of the receptors. The potential therapeutic value offered from RAR modulation provides the impetus to identify novel ligands based on unique scaffolds that may offer improved toxicity and pharmacokinetic profiles. Here we describe the identification of an atypical RAR inverse agonist that represents the first non-acid, non-retinoid direct modulator of RAR receptor subfamily. SR-0065 functions as a pan-RAR inverse agonist suppressing the basal activity of RARα, RARβ, and RARγ, as well as inhibiting agonist-induced RAR activity. SR-0065 treatment enhanced receptor interaction with a peptide representative of the corepressor SMRT, and in cells SR-0065 enhances recruitment of SMRT to the promoter of the RARγ dependent gene, Cyp26A1. The acid form of SR-0065, SR-1758, was inactive in all assays. Thus, SR-0065 represents a new class of non-acid, non-retinoid RAR modulator that may be used as a point to initiate development of improved RAR-targeted drugs.
视黄醇是维生素 A 的有效形式,参与广泛的生理过程,视黄醇的药理学效应主要通过视黄酸受体 (RARs) 和视黄醛受体 (RXRs) 介导。一些天然和合成的 RAR 调节剂已被证明对多种治疗适应症具有临床应用价值,包括癌症、银屑病和糖尿病。不幸的是,这些药物会导致许多严重的副作用。大多数合成的视黄醇配体基于视黄醇支架,因此与天然配体具有相似性,所有以前公开的 RAR 配体都具有羧酸,在受体的配体结合域内形成关键的离子桥。RAR 调节所提供的潜在治疗价值促使我们基于独特的支架来识别新型配体,这些配体可能具有改善的毒性和药代动力学特征。在这里,我们描述了一种非典型的 RAR 反向激动剂的鉴定,它代表了第一个非酸、非视黄醇的 RAR 受体亚家族直接调节剂。SR-0065 作为一种 pan-RAR 反向激动剂,抑制 RARα、RARβ 和 RARγ 的基础活性,以及抑制激动剂诱导的 RAR 活性。SR-0065 处理增强了受体与代表核心抑制因子 SMRT 的肽的相互作用,并且在细胞中,SR-0065 增强了 SMRT 募集到 RARγ 依赖性基因 Cyp26A1 启动子的能力。SR-0065 的酸形式 SR-1758 在所有检测中均无活性。因此,SR-0065 代表了一类新的非酸、非视黄醇的 RAR 调节剂,可作为开发改进的 RAR 靶向药物的起点。