Robinson Marin S, Zhao Min, Zack Lindsay, Brindley Christine, Portz Lillian, Quarterman Matthew, Long Xiufen, Herckes Pierre
Department of Chemistry and Biochemistry, Northern Arizona University, Flagstaff, AZ 86011.
Atmos Environ (1994). 2011 Apr;45(12):2087-2094. doi: 10.1016/j.atmosenv.2011.01.051.
Prescribed burning, in combination with mechanical thinning, is a successful method for reducing heavy fuel loads from forest floors and thereby lowering the risk of catastrophic wildfire. However, an undesirable consequence of managed fire is the production of fine particulate matter or PM(2.5) (particles ≤2.5 µm in aerodynamic diameter). Wood-smoke particulate data from 21 prescribed burns are described, including results from broadcast and slash-pile burns. All PM(2.5) samples were collected in situ on day 1 (ignition) or day 2. Samples were analyzed for mass, polycyclic aromatic hydrocarbons (PAHs), inorganic elements, organic carbon (OC), and elemental carbon (EC). Results were characteristic of low intensity, smoldering fires. PM(2.5) concentrations varied from 523 to 8357 µg m(-3) and were higher on day 1. PAH weight percents (19 PAHs) were higher in slash-pile burns (0.21 ± 0.08% OC) than broadcast burns (0.07 ± 0.03% OC). The major elements were K, Cl, S, and Si. OC and EC values averaged 66 ± 7 and 2.8 ± 1.4% PM(2.5), respectively, for all burns studied, in good agreement with literature values for smoldering fires.
规定火烧结合机械疏伐是一种成功的方法,可减少森林地面的重燃料负荷,从而降低灾难性野火的风险。然而,计划性火烧的一个不良后果是产生细颗粒物或PM(2.5)(空气动力学直径≤2.5微米的颗粒)。本文描述了来自21次规定火烧的木烟颗粒数据,包括大面积火烧和堆积枝桠火烧的结果。所有PM(2.5)样本均在第1天(点火)或第2天现场采集。对样本进行了质量、多环芳烃(PAHs)、无机元素、有机碳(OC)和元素碳(EC)分析。结果显示为低强度阴燃火灾的特征。PM(2.5)浓度在523至8357微克/立方米之间变化,且在第1天更高。堆积枝桠火烧中PAH重量百分比(19种PAHs)(0.21±0.08% OC)高于大面积火烧(0.07±0.03% OC)。主要元素为钾、氯、硫和硅。在所研究的所有火烧中,OC和EC值分别平均占PM(2.5)的66±7%和2.8±1.4%,与阴燃火灾的文献值高度一致。