Department of Chemistry & Biochemistry, Presidency University, Kolkata 700 073, India.
J Fluoresc. 2011 Nov;21(6):2123-32. doi: 10.1007/s10895-011-0913-4. Epub 2011 Jul 12.
We have investigated the localization and environment of tryptophan residues in different quaternary and conformational states (tetrameric, dimeric, monomeric and unfolded) of metallized and demetallized concanavalin A (ConA) by selective chemical modification, fluorescence, and phosphorescence. ConA has four tryptophan residues (Trp 40, Trp 88, Trp 109 and Trp 182) per subunit. The pattern of oxidation by N-bromosuccinimide (NBS) shows that NBS modifies, in dimer, only Trp 182 which remains inaccessible in tetramer, two (Trp 88 along with Trp 182) in monomer, all four in unfolded form in presence of EDTA, and three (possibly Trp 40 along with Trp 88 and Trp 182) in unfolded form from native or remetallized ConA. Utilizing wavelength-selective fluorescence approach, we have observed a red edge excitation shift (REES) of 6-8 nm for tetramer and dimer. A more pronounced REES (11 nm) is observed for oxidized monomer compared to REES (3 nm) for unoxidized species. Acrylamide quenching shows the Stern-Volmer constant (K(SV)) for dimer, monomer, unfolded ConA and unfolded apo-ConA being 3.8, 5.2, 12.8, 14.0 M(-1), respectively. Phosphorescence studies at 77 K give more structured spectra, with two (0,0) bands at 406.2 (weak) and 413.2 nm for tetramer. However, a single (0,0) band appears at 413.2 for dimer and 412.6 nm for monomer, while the (0,0) band of the oxidized monomer is red shifted to 414.4 nm. These results may provide important insight into subtlety of organization and environment of tryptophans in the context of folding and structural studies of oligomeric proteins including lectins.
我们通过选择性化学修饰、荧光和磷光研究了色氨酸残基在金属化和去金属化的伴刀豆球蛋白 A(ConA)的不同四元体和构象状态(四聚体、二聚体、单体和未折叠)中的定位和环境。ConA 每个亚基含有四个色氨酸残基(Trp40、Trp88、Trp109 和 Trp182)。N-溴代丁二酰亚胺(NBS)的氧化模式表明,NBS 在二聚体中仅修饰 Trp182,而在四聚体中 Trp182 是不可接近的,在单体中修饰两个(Trp88 与 Trp182),在存在 EDTA 时在未折叠形式中修饰所有四个,在天然或再金属化 ConA 的未折叠形式中修饰三个(可能是 Trp40 与 Trp88 和 Trp182)。利用波长选择性荧光方法,我们观察到四聚体和二聚体的红色边缘激发位移(REES)为 6-8nm。与未氧化的物种相比,氧化的单体观察到更明显的 REES(11nm)。丙烯酰胺猝灭表明二聚体、单体、未折叠 ConA 和未折叠 apo-ConA 的 Stern-Volmer 常数(KSV)分别为 3.8、5.2、12.8 和 14.0M(-1)。在 77K 下进行磷光研究可得到更具结构的光谱,四聚体在 406.2(弱)和 413.2nm 处有两个(0,0)带。然而,二聚体出现一个(0,0)带,在 413.2nm 处,单体在 412.6nm 处出现一个(0,0)带,而氧化的单体的(0,0)带则红移至 414.4nm。这些结果可能为折叠和寡聚蛋白(包括凝集素)结构研究中色氨酸的细微组织和环境提供重要的见解。