Department of Civil and Environmental Engineering, University of Hawaii at Manoa, Honolulu, Hawaii, 96822 USA.
Environ Sci Technol. 2011 Oct 15;45(20):8683-90. doi: 10.1021/es2019115. Epub 2011 Sep 26.
This study investigated the flux stability of select chemical and biological sewage markers, including caffeine, total nitrogen (TN), total suspended solids (TSS), E. coli, and enterococci, and their suitability in assessing the severity of rainfall-derived infiltration and inflow (RDII) in a residential sewershed. To quantify and compare marker flux stability, concentrations of the candidate markers in two dry-weather periods were determined and the one-day lag autocorrelation coefficients (r) of their mass fluxes were calculated. TN (r = 0.82-0.88) exhibited higher and more consistent flux stability than TSS (r = 0.49-0.82), caffeine (r = 0.56-0.58), E. coli (r = 0.36-0.87), and enterococci (by culture; r = 0.40-0.52), all of which except enterococci by qPCR (r = -0.10-0.21) showed significant autocorrelation. Sewage flows and marker concentrations were also monitored in two wet-weather periods, and the severity of RDII (R(RDII)) were calculated using either flow measurements or marker concentrations independently. Corresponding to its outstanding flux stability, R(RDII) values estimated by TN predicted all severe RDII instances and gave the highest and most consistent correlation (r = 0.74-0.78) among the different sewage markers. Overall, the study illustrated the feasibility of using the flux stability of sewage markers in assessing the severity of RDII and thereby deterioration levels in sewer systems.
本研究调查了包括咖啡因、总氮(TN)、总悬浮固体(TSS)、大肠杆菌和肠球菌在内的选定化学和生物污水标志物的通量稳定性,以及它们在评估住宅污水流域中降雨衍生渗透和流入(RDII)严重程度的适用性。为了量化和比较标记物通量稳定性,确定了两个干期候选标记物的浓度,并计算了它们质量通量的一天滞后自相关系数(r)。TN(r = 0.82-0.88)表现出比 TSS(r = 0.49-0.82)、咖啡因(r = 0.56-0.58)、大肠杆菌(r = 0.36-0.87)和肠球菌(通过培养;r = 0.40-0.52)更高且更一致的通量稳定性,除了通过 qPCR 的肠球菌(r = -0.10-0.21)之外,所有这些标记物的通量都显示出显著的自相关性。在两个湿期也监测了污水流量和标记物浓度,并使用流量测量或标记物浓度独立计算 RDII 的严重程度(R(RDII))。与出色的通量稳定性相对应,TN 估算的 R(RDII)值预测了所有严重的 RDII 实例,并在不同的污水标记物之间给出了最高和最一致的相关性(r = 0.74-0.78)。总体而言,该研究说明了使用污水标记物通量稳定性评估 RDII 严重程度以及因此评估污水系统恶化程度的可行性。