Institut für Physik und Astronomie, Universität Potsdam, Karl-Liebknecht-Str. 24∕25, 14476 Potsdam, Germany.
J Chem Phys. 2011 Oct 28;135(16):164901. doi: 10.1063/1.3656248.
We report spatiotemporal chaos in the Oregonator model of the Belousov-Zhabotinsky reaction. Spatiotemporal chaos spontaneously develops in a regime, where the underlying local dynamics show stable limit cycle oscillations (diffusion-induced turbulence). We show that spatiotemporal chaos can be suppressed by a unidirectional flow in the system. With increasing flow velocity, we observe a transition scenario from spatiotemporal chaos via a regime of travelling waves to a stationary steady state. At large flow velocities, we recover the known regime of flow distributed oscillations.
我们报告了 Belousov-Zhabotinsky 反应的 Oregonator 模型中的时空混沌。在局部动力学表现出稳定的极限环振荡(扩散诱导的湍流)的区域,时空混沌会自发地发展。我们表明,通过系统中的单向流可以抑制时空混沌。随着流速的增加,我们观察到从时空混沌到行波的转变情景,再到稳定的静态状态。在较大的流速下,我们恢复了已知的流速分布振荡区域。