Department of Chemistry, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA.
J Phys Chem B. 2011 Dec 29;115(51):15332-8. doi: 10.1021/jp2046867. Epub 2011 Dec 2.
The thermal stability and folding kinetics of a series of 15-residue β-hairpins with a common Type I [3:5] NPDG turn were studied using Fourier transform infrared spectroscopy (FTIR) and laser-induced temperature jump (T-jump) with infrared detection, respectively. Mutations at positions 3, 5, or 13 in the peptide sequence SEXYXNPDGTWTXTE, where X represents the position of mutation, were performed to study the roles of hydrophobic interactions in determining the thermodynamic and kinetic properties of β-hairpin folding. The thermal stability studies show a broad thermal folding/unfolding transition for all the peptides. T-jump studies indicate that these β-hairpin peptides fold in less than 2 μs. In addition, both folding and unfolding rate constants decrease with increasing strength of hydrophobic interactions. Kinetically, the hydrophobic interactions have more significant influence on the unfolding rate than the folding rate. Φ-value analysis indicates that the hydrophobic interactions between the side chains are mainly formed at the latter part of the transition-state region during the folding process. In summary, the results suggest that the formation of the native structure of these β-hairpins depends on the correct topology of the hydrophobic cluster. Besides the formation of the turn region as a key process for folding as suggested by previous studies, a hydrophobic collapse process may also play a crucial role during β-hairpin folding.
使用傅里叶变换红外光谱(FTIR)和激光诱导温度跃变(T-jump)结合红外检测,分别研究了一系列具有共同 I 型 [3:5] NPDG 转角的 15 残基β发夹的热稳定性和折叠动力学。在肽序列 SEXYXNPDGTWTXTE 中,在位置 3、5 或 13 处进行突变,以研究疏水相互作用在确定β发夹折叠热力学和动力学性质中的作用,X 代表突变位置。热稳定性研究表明所有肽都有广泛的热折叠/去折叠转变。T-jump 研究表明这些β发夹肽在不到 2 μs 的时间内折叠。此外,折叠和去折叠速率常数都随疏水相互作用强度的增加而降低。动力学研究表明,疏水相互作用对去折叠速率的影响比对折叠速率的影响更大。Φ 值分析表明,在折叠过程中,疏水相互作用主要在过渡态区域的后一部分形成。总之,结果表明这些β发夹的天然结构的形成取决于疏水簇的正确拓扑。除了先前研究表明的转角区域的形成是折叠的关键过程外,疏水塌陷过程也可能在β发夹折叠过程中发挥关键作用。