Department of Physics and Astronomy, The University of Tennessee, Knoxville, Tennessee 37996-1200, USA.
Nat Commun. 2011 Dec 6;2:580. doi: 10.1038/ncomms1573.
The parent compounds of iron pnictide superconductors are bad metals with a collinear antiferromagnetic structure and Néel temperatures below 220 K. Although alkaline iron selenide A(y)Fe(1.6+x)Se(2) (A=K, Rb, Cs) superconductors are isostructural with iron pnictides, in the vicinity of the undoped limit they are insulators, forming a block antiferromagnetic order and having Néel temperatures of roughly 500 K. Here we show that the spin waves of the insulating antiferromagnet Rb(0.89)Fe(1.58)Se(2) can be accurately described by a local moment Heisenberg Hamiltonian. A fitting analysis of the spin wave spectra reveals that the next-nearest neighbour couplings in Rb(0.89)Fe(1.58)Se(2), (Ba,Ca,Sr)Fe(2)As(2), and Fe(1.05)Te are of similar magnitude. Our results suggest a common origin for the magnetism of all the Fe-based superconductors, despite having different ground states and antiferromagnetic orderings.
铁磷化物超导体的母体化合物是具有斜交反铁磁结构和低于 220K 的尼尔温度的不良金属。尽管碱性铁硒化物 A(y)Fe(1.6+x)Se(2)(A=K、Rb、Cs)与铁磷化物具有同构性,但在未掺杂极限附近,它们是绝缘体,形成块体反铁磁有序,尼尔温度约为 500K。在这里,我们表明绝缘反铁磁体 Rb(0.89)Fe(1.58)Se(2)的自旋波可以通过局域矩海森堡哈密顿量准确描述。对自旋波谱的拟合分析表明,Rb(0.89)Fe(1.58)Se(2)、(Ba,Ca,Sr)Fe(2)As(2)和 Fe(1.05)Te 中的最近邻和次近邻耦合具有相似的大小。尽管具有不同的基态和反铁磁有序,但我们的结果表明所有铁基超导体的磁性具有共同的起源。