Biomolecular Mass Spectrometry and Proteomics Group, Utrecht Institute for Pharmaceutical Sciences and Bijvoet Center for Biomolecular Research, Utrecht University, Padualaan 8, 3584 CH Utrecht, The Netherlands.
Proc Natl Acad Sci U S A. 2012 Jan 10;109(2):407-12. doi: 10.1073/pnas.1108399108. Epub 2011 Dec 22.
Mass spectrometry (MS)-based proteome analysis relies heavily on the presence of complete protein databases. Such a strategy is extremely powerful, albeit not adequate in the analysis of unpredicted postgenome events, such as posttranslational modifications, which exponentially increase the search space. Therefore, it is of interest to explore "database-free" approaches. Here, we sampled the ostrich and human proteomes with a method facilitating de novo sequencing, utilizing the protease Lys-N in combination with electron transfer dissociation. By implementing several validation steps, including the combined use of collision-induced dissociation/electron transfer dissociation data and a cross-validation with conventional database search strategies, we identified approximately 2,500 unique de novo peptide sequences from the ostrich sample with over 900 peptides generating full backbone sequence coverage. This dataset allowed the appropriate positioning of ostrich in the evolutionary tree. The described database-free sequencing approach is generically applicable and has great potential in important proteomics applications such as in the analysis of variable parts of endogenous antibodies or proteins modified by a plethora of complex posttranslational modifications.
基于质谱(MS)的蛋白质组分析严重依赖于完整的蛋白质数据库的存在。这种策略非常强大,尽管不足以分析未预测的后基因组事件,如翻译后修饰,这些修饰会使搜索空间呈指数级增长。因此,探索“无数据库”方法很有意义。在这里,我们使用一种促进从头测序的方法对鸵鸟和人类蛋白质组进行了采样,该方法利用了蛋白酶 Lys-N 并结合了电子转移解离。通过实施包括碰撞诱导解离/电子转移解离数据的联合使用以及与传统数据库搜索策略的交叉验证在内的几个验证步骤,我们从鸵鸟样本中鉴定出了大约 2500 个独特的从头肽序列,其中超过 900 个肽生成了完整的骨架序列覆盖。该数据集允许将鸵鸟在进化树上的正确定位。所描述的无数据库测序方法具有通用性,并且在重要的蛋白质组学应用中具有很大的潜力,例如分析内源性抗体的可变部分或受大量复杂翻译后修饰修饰的蛋白质。