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Mode-coupling glass transition in a fluid confined by a periodic potential.

作者信息

Nandi Saroj Kumar, Bhattacharyya Sarika Maitra, Ramaswamy Sriram

机构信息

Centre for Condensed Matter Theory, Department of Physics, Indian Institute of Science, Bangalore 560 012, India.

出版信息

Phys Rev E Stat Nonlin Soft Matter Phys. 2011 Dec;84(6 Pt 1):061501. doi: 10.1103/PhysRevE.84.061501. Epub 2011 Dec 2.

Abstract

We show that a fluid under strong spatially periodic confinement displays a glass transition within mode-coupling theory at a much lower density than the corresponding bulk system. We use fluctuating hydrodynamics, with confinement imposed through a periodic potential whose wavelength plays an important role in our treatment. To make the calculation tractable we implement a detailed calculation in one dimension. Although we do not expect simple 1d fluids to show a glass transition, our results are indicative of the behavior expected in higher dimensions. In a certain region of parameter space we observe a three-step relaxation reported recently in computer simulations [S. H. Krishnan, Ph.D. thesis, Indian Institute of Science (2005); Kim et al., Eur. Phys. J. Special Topics 189, 135 (2010)] and a glass-glass transition. We compare our results to those of Krakoviack [Phys. Rev. E 75, 031503 (2007)] and Lang et al. [Phys. Rev. Lett. 105, 125701 (2010)].

摘要

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