Li Jin-Jin, Zhu Ka-Di
Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics, Shanghai Jiao Tong University, 800 Dong Chuan Road, Shanghai 200240, China.
Nanoscale Res Lett. 2012 Feb 16;7(1):133. doi: 10.1186/1556-276X-7-133.
We theoretically investigate coherent optical spectroscopy of a biological semiconductor quantum dot (QD) coupled to DNA molecules. Coupling with DNAs, the linear optical responses of the peptide QDs will be enhanced significantly in the simultaneous presence of two optical fields. Based on this technique, we propose a scheme to measure the vibrational frequency of DNA and the coupling strength between peptide QD and DNA in all-optical domain. Distinct with metallic quantum dot, biological QD is non-toxic and pollution-free to environment, which will contribute to clinical medicine experiments. This article leads people to know more about the optical behaviors of DNAs-quantum dot system, with the currently popular pump-probe technique.
我们从理论上研究了与DNA分子耦合的生物半导体量子点(QD)的相干光学光谱。与DNA耦合时,在两个光场同时存在的情况下,肽量子点的线性光学响应将显著增强。基于该技术,我们提出了一种在全光域中测量DNA振动频率以及肽量子点与DNA之间耦合强度的方案。与金属量子点不同,生物量子点对环境无毒且无污染,这将有助于临床医学实验。本文利用当前流行的泵浦-探测技术,使人们更多地了解DNA-量子点系统的光学行为。