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通过热梯度对纳米颗粒进行操控。

Nanoparticle manipulation by thermal gradient.

作者信息

Wei Ning, Wang Hui-Qiong, Zheng Jin-Cheng

机构信息

Department of Physics and Institute of Theoretical Physics and Astrophysics, Xiamen University, Xiamen, 361005, China.

出版信息

Nanoscale Res Lett. 2012 Feb 26;7(1):154. doi: 10.1186/1556-276X-7-154.

DOI:10.1186/1556-276X-7-154
PMID:22364240
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC3306267/
Abstract

A method was proposed to manipulate nanoparticles through a thermal gradient. The motion of a fullerene molecule enclosed inside a (10, 10) carbon nanotube with a thermal gradient was studied by molecular dynamics simulations. We created a one-dimensional potential valley by imposing a symmetrical thermal gradient inside the nanotube. When the temperature gradient was large enough, the fullerene sank into the valley and became trapped. The escaping velocities of the fullerene were evaluated based on the relationship between thermal gradient and thermophoretic force. We then introduced a new way to manipulate the position of nanoparticles by translating the position of thermostats with desirable thermal gradients. Compared to nanomanipulation using a scanning tunneling microscope or an atomic force microscope, our method for nanomanipulation has a great advantage by not requiring a direct contact between the probe and the object.

摘要

提出了一种通过热梯度操纵纳米颗粒的方法。通过分子动力学模拟研究了在具有热梯度的(10, 10)碳纳米管内的富勒烯分子的运动。我们通过在纳米管内施加对称热梯度创建了一个一维势谷。当温度梯度足够大时,富勒烯沉入谷中并被困住。基于热梯度与热泳力之间的关系评估了富勒烯的逃逸速度。然后,我们引入了一种通过平移具有所需热梯度的恒温器位置来操纵纳米颗粒位置的新方法。与使用扫描隧道显微镜或原子力显微镜进行纳米操纵相比,我们的纳米操纵方法具有很大优势,因为它不需要探针与物体直接接触。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9184/3306267/118adc8d2a33/1556-276X-7-154-3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9184/3306267/e8a6f692a2a5/1556-276X-7-154-1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9184/3306267/118adc8d2a33/1556-276X-7-154-3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9184/3306267/e8a6f692a2a5/1556-276X-7-154-1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9184/3306267/118adc8d2a33/1556-276X-7-154-3.jpg

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本文引用的文献

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Knitted graphene-nanoribbon sheet: a mechanically robust structure.编织石墨烯纳米带片:一种机械坚固的结构。
Nanoscale. 2012 Feb 7;4(3):785-91. doi: 10.1039/c1nr11200g. Epub 2011 Dec 15.
2
Strain engineering of thermal conductivity in graphene sheets and nanoribbons: a demonstration of magic flexibility.石墨烯片和纳米带中热导率的应变工程:神奇柔韧性的展示。
Nanotechnology. 2011 Mar 11;22(10):105705. doi: 10.1088/0957-4484/22/10/105705. Epub 2011 Feb 2.
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Thermally driven molecular linear motors: a molecular dynamics study.热驱动分子线性马达:分子动力学研究。
Nanoscale Res Lett. 2020 Oct 28;15(1):203. doi: 10.1186/s11671-020-03434-6.
J Chem Phys. 2009 Dec 28;131(24):241104. doi: 10.1063/1.3281642.
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Thermal gradient induced actuation in double-walled carbon nanotubes.热梯度诱导双壁碳纳米管的致动。
Nanotechnology. 2009 Dec 9;20(49):495503. doi: 10.1088/0957-4484/20/49/495503. Epub 2009 Nov 6.
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Strain controlled thermomutability of single-walled carbon nanotubes.单壁碳纳米管的应变控制热变性
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Water transport inside a single-walled carbon nanotube driven by a temperature gradient.由温度梯度驱动的单壁碳纳米管内的水传输。
Nanotechnology. 2009 Feb 4;20(5):055708. doi: 10.1088/0957-4484/20/5/055708. Epub 2009 Jan 12.
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Thermophoretic motion of water nanodroplets confined inside carbon nanotubes.限制在碳纳米管内的水纳米液滴的热泳运动。
Nano Lett. 2009 Jan;9(1):66-71. doi: 10.1021/nl802429s.
8
A molecular linear motor consisting of carbon nanotubes.
Nano Lett. 2009 Jan;9(1):62-5. doi: 10.1021/nl802323n.
9
A freight train of nanotubes for cargo transport on the nanoscale.一列用于纳米级货物运输的纳米管“货运列车”。
Angew Chem Int Ed Engl. 2008;47(45):8565-6. doi: 10.1002/anie.200803021.
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Subnanometer motion of cargoes driven by thermal gradients along carbon nanotubes.货物在沿碳纳米管的热梯度驱动下的亚纳米级运动。
Science. 2008 May 9;320(5877):775-8. doi: 10.1126/science.1155559. Epub 2008 Apr 10.