Thakur P, Ballard S, Nelson R
Carlsbad Environmental Monitoring & Research Center, 1400 University Drive, Carlsbad, New Mexico-88220, USA.
J Environ Monit. 2012 May;14(5):1317-24. doi: 10.1039/c2em11011c. Epub 2012 Mar 29.
The release of radioactivity into the atmosphere from the damaged Fukushima Daiichi nuclear power plant started on March 12th, 2011. Among the various radionuclides released, iodine -131 ((131)I) and cesium isotopes ((137)Cs and (134)Cs) were transported across the Pacific Ocean and reached the United States on 17-18 March 2011. Consequently, an elevated level of fission products (131)I, (132)I, (132)Te, (134)Cs and (137)Cs were detected in air, water, and milk samples collected across the United States between March 17 and April 4, 2011. The continuous monitoring of activities over a period of 25 days and spatial variations across more than 100 sampling locations in the United States made it possible to characterize the contaminated air masses. For the entire period, the highest detected activity values ranged from less than 1 m Bq m(-3) to 31 m Bq m(-3) for the particulate (131)I, and up to 96 m Bq m(-3) for the gaseous (131)I fraction.
2011年3月12日,受损的福岛第一核电站开始向大气中释放放射性物质。在释放出的各种放射性核素中,碘 -131(¹³¹I)和铯同位素(¹³⁷Cs和¹³⁴Cs)跨越太平洋,并于2011年3月17 - 18日抵达美国。因此,在2011年3月17日至4月4日期间,在美国各地采集的空气、水和牛奶样本中检测到裂变产物¹³¹I、¹³²I、¹³²Te、¹³⁴Cs和¹³⁷Cs的含量升高。对美国100多个采样点超过25天的活度进行持续监测以及空间变化监测,使得确定受污染气团的特征成为可能。在整个期间,检测到的最高活度值范围为:颗粒态¹³¹I小于1 mBq m⁻³至31 mBq m⁻³,气态¹³¹I部分高达96 mBq m⁻³。