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石墨烯中关联导致的光学自能。

Optical self-energy in graphene due to correlations.

机构信息

Department of Physics, Sungkyunkwan University, Suwon, Gyeonggi-do, Republic of Korea.

出版信息

J Phys Condens Matter. 2012 Jun 20;24(24):245601. doi: 10.1088/0953-8984/24/24/245601. Epub 2012 May 18.

Abstract

In highly correlated systems one can define an optical self-energy in analogy to its quasiparticle (QP) self-energy counterpart. This quantity provides useful information on the nature of the excitations involved in inelastic scattering processes. Here we calculate the self-energy of the intraband optical transitions in graphene originating in the electron-electron interaction (EEI) as well as electron-phonon interaction (EPI). Although optics involves an average over all momenta (k) of the charge carriers, the structure in the optical self-energy is nevertheless found to mirror mainly that of the corresponding quasiparticles for k equal to or near the Fermi momentum k(F). Consequently, plasmaronic structures which are associated with momenta near the Dirac point at k = 0 are not important in the intraband optical response. While the structure of the electron-phonon interaction (EPI) reflects the sharp peaks of the phonon density of states, the excitation spectrum associated with the electron-electron interaction is in comparison structureless and flat and extends over an energy range which scales linearly with the value of the chemical potential. We introduce a method whereby detailed quantitative information on such excitation spectra can be extracted from optical data. Modulations seen on the edge of the interband optical conductivity as it rises towards its universal background value are traced to structure in the quasiparticle self-energies around k(F) of the lower Dirac cone associated with the occupied states.

摘要

在高度相关的系统中,可以类比其准粒子(QP)自能来定义光学自能。这个量提供了关于非弹性散射过程中涉及的激发性质的有用信息。在这里,我们计算了起源于电子-电子相互作用(EEI)和电子-声子相互作用(EPI)的石墨烯中带内光跃迁的自能。虽然光学涉及到载流子所有动量(k)的平均值,但在光学自能中的结构仍然发现主要反映了相应准粒子的结构,对于等于或接近费米动量 k(F)的 k。因此,与 k = 0 处的狄拉克点附近动量相关的等离激元结构在带内光学响应中并不重要。虽然电子-声子相互作用(EPI)的结构反映了声子态密度的尖锐峰,但与电子-电子相互作用相关的激发谱与结构无关且平坦,并扩展到与化学势的线性比例的能量范围。我们引入了一种方法,通过该方法可以从光学数据中提取出有关这种激发谱的详细定量信息。随着它向普遍背景值上升,在带间光导率的边缘看到的调制可以追溯到与占据态相关的较低狄拉克锥的费米动量 k(F)周围准粒子自能的结构。

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