JILA, University of Colorado at Boulder, Boulder, CO 80309, USA.
Science. 2012 Jun 8;336(6086):1287-91. doi: 10.1126/science.1218497.
High-harmonic generation (HHG) traditionally combines ~100 near-infrared laser photons to generate bright, phase-matched, extreme ultraviolet beams when the emission from many atoms adds constructively. Here, we show that by guiding a mid-infrared femtosecond laser in a high-pressure gas, ultrahigh harmonics can be generated, up to orders greater than 5000, that emerge as a bright supercontinuum that spans the entire electromagnetic spectrum from the ultraviolet to more than 1.6 kilo-electron volts, allowing, in principle, the generation of pulses as short as 2.5 attoseconds. The multiatmosphere gas pressures required for bright, phase-matched emission also support laser beam self-confinement, further enhancing the x-ray yield. Finally, the x-ray beam exhibits high spatial coherence, even though at high gas density the recolliding electrons responsible for HHG encounter other atoms during the emission process.
高次谐波产生(HHG)传统上结合了约 100 个近红外激光光子,当来自许多原子的发射建设性地相加时,产生明亮、相匹配的极紫外光束。在这里,我们表明,通过在高压气体中引导中红外飞秒激光,可以产生超高次谐波,其阶数超过 5000,作为明亮的超连续体出现,覆盖从紫外线到超过 1600 电子伏特的整个电磁光谱,从而在理论上允许产生短至 2.5 飞秒的脉冲。用于明亮、相匹配发射的多大气压也支持激光束自约束,进一步提高了 X 射线的产量。最后,X 射线束表现出高的空间相干性,即使在高气体密度下,负责 HHG 的再碰撞电子在发射过程中也会与其他原子相遇。