Diamond Light Source Ltd, Chilton, Didcot, Oxfordshire OX11 0DE, UK.
J Phys Condens Matter. 2012 Jul 25;24(29):294204. doi: 10.1088/0953-8984/24/29/294204.
We report on magnetic susceptibility and specific heat measurements of the cubic helimagnet FeGe in external magnetic fields and temperatures near the onset of long-range magnetic order at TC = 278.2(3) K. Pronounced anomalies in the field-dependent χac(H) data as well as in the corresponding imaginary part χ''ac(H) reveal a precursor region around TC in the magnetic phase diagram. The occurrence of a maximum at T0 = 279.6 K in the zero-field specific heat data indicates a second-order transition into a magnetically ordered state. A shoulder evolves above this maximum as a magnetic field is applied. The field dependence of both features coincides with crossover lines from the field-polarized to the paramagnetic state deduced from χac(T) at constant magnetic fields. The experimental findings are analyzed within the standard Dzyaloshinskii theory for cubic helimagnets. The remarkable multiplicity of modulated precursor states and the complexity of the magnetic phase diagram near the magnetic ordering are explained by the change of the character of solitonic inter-core interactions and the onset of specific confined chiral modulations in this area.
我们报告了立方海姆磁体 FeGe 在外部磁场和接近 TC=278.2(3) K 的长程磁有序起始温度下的磁化率和比热测量结果。在磁场相关的 χac(H)数据以及相应的虚部 χ''ac(H)中,明显的异常揭示了磁相图中 TC 周围的前驱区。在零场比热数据中 T0=279.6 K 处出现最大值表明存在向磁有序态的二级相变。当施加磁场时,在该最大值上方出现一个肩峰。这两个特征的磁场依赖性与从 χac(T) 在恒磁场下推断出的从极化场到顺磁态的交叉线一致。实验结果在立方海姆磁体的标准 Dzyaloshinskii 理论内进行了分析。调制前驱态的显著多重性和磁有序附近磁相图的复杂性可以通过核心间相互作用的孤子特征的变化以及该区域中特定受限手性调制的出现来解释。