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用于能源和环境应用的多功能氧化物基复合纳米结构的分级组装

Hierarchical assembly of multifunctional oxide-based composite nanostructures for energy and environmental applications.

作者信息

Gao Pu-Xian, Shimpi Paresh, Gao Haiyong, Liu Caihong, Guo Yanbing, Cai Wenjie, Liao Kuo-Ting, Wrobel Gregory, Zhang Zhonghua, Ren Zheng, Lin Hui-Jan

机构信息

Nanomaterials Science Laboratory, Department of Chemical, Materials and Biomolecular Engineering & Institute of Materials Science, University of Connecticut, Storrs, CT 06269, USA.

出版信息

Int J Mol Sci. 2012;13(6):7393-7423. doi: 10.3390/ijms13067393. Epub 2012 Jun 15.

DOI:10.3390/ijms13067393
PMID:22837702
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC3397534/
Abstract

Composite nanoarchitectures represent a class of nanostructured entities that integrates various dissimilar nanoscale building blocks including nanoparticles, nanowires, and nanofilms toward realizing multifunctional characteristics. A broad array of composite nanoarchitectures can be designed and fabricated, involving generic materials such as metal, ceramics, and polymers in nanoscale form. In this review, we will highlight the latest progress on composite nanostructures in our research group, particularly on various metal oxides including binary semiconductors, ABO(3)-type perovskites, A(2)BO(4) spinels and quaternary dielectric hydroxyl metal oxides (AB(OH)(6)) with diverse application potential. Through a generic template strategy in conjunction with various synthetic approaches- such as hydrothermal decomposition, colloidal deposition, physical sputtering, thermal decomposition and thermal oxidation, semiconductor oxide alloy nanowires, metal oxide/perovskite (spinel) composite nanowires, stannate based nanocompostes, as well as semiconductor heterojunction-arrays and networks have been self-assembled in large scale and are being developed as promising classes of composite nanoarchitectures, which may open a new array of advanced nanotechnologies in solid state lighting, solar absorption, photocatalysis and battery, auto-emission control, and chemical sensing.

摘要

复合纳米结构是一类纳米结构实体，它集成了各种不同的纳米级构建块，包括纳米颗粒、纳米线和纳米薄膜，以实现多功能特性。可以设计和制造各种各样的复合纳米结构，涉及纳米级形式的通用材料，如金属、陶瓷和聚合物。在这篇综述中，我们将重点介绍我们研究小组在复合纳米结构方面的最新进展，特别是在各种金属氧化物方面，包括具有不同应用潜力的二元半导体、ABO(3)型钙钛矿、A(2)BO(4)尖晶石和四元介电羟基金属氧化物(AB(OH)(6))。通过通用模板策略结合各种合成方法，如热分解、胶体沉积、物理溅射、热分解和热氧化，半导体氧化物合金纳米线、金属氧化物/钙钛矿(尖晶石)复合纳米线、锡酸盐基纳米复合材料以及半导体异质结阵列和网络已被大规模自组装，并正在被开发为有前景的复合纳米结构类别，这可能会在固态照明、太阳能吸收、光催化和电池、汽车排放控制以及化学传感等领域开启一系列新的先进纳米技术。

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