School of Engineering, University of California, 5200 Lake Road, Merced, California 95343, United States.
Environ Sci Technol. 2012 Oct 2;46(19):10835-41. doi: 10.1021/es301851x. Epub 2012 Sep 20.
Although biofuels present an opportunity for renewable energy production, significant land-use change resulting from biofuels may contribute to negative environmental, economic, and social impacts. Here we examined non-GHG air pollution impacts from both indirect and direct land-use change caused by the anticipated expansion of Brazilian biofuels production. We synthesized information on fuel loading, combustion completeness, and emission factors, and developed a spatially explicit approach with uncertainty and sensitivity analyses to estimate air pollution emissions. The land-use change emissions, ranging from 6.7 to 26.4 Tg PM(2.5), were dominated by deforestation burning practices associated with indirect land-use change. We also found Brazilian sugar cane ethanol and soybean biodiesel including direct and indirect land-use change effects have much larger life-cycle emissions than conventional fossil fuels for six regulated air pollutants. The emissions magnitude and uncertainty decrease with longer life-cycle integration periods. Results are conditional to the single LUC scenario employed here. After LUC uncertainty, the largest source of uncertainty in LUC emissions stems from the combustion completeness during deforestation. While current biofuels cropland burning policies in Brazil seek to reduce life-cycle emissions, these policies do not address the large emissions caused by indirect land-use change.
虽然生物燃料为可再生能源生产提供了机会,但生物燃料导致的土地利用方式的重大变化可能会对环境、经济和社会造成负面影响。在这里,我们研究了由于巴西生物燃料生产预期扩张而导致的间接和直接土地利用变化对非 GHG 空气污染的影响。我们综合了燃料负荷、燃烧完全度和排放因子的信息,并开发了一种具有不确定性和敏感性分析的空间明确方法来估算空气污染排放。土地利用变化排放量在 6.7 到 26.4 兆吨 PM(2.5)之间,主要来自与间接土地利用变化相关的毁林燃烧实践。我们还发现,巴西甘蔗乙醇和大豆生物柴油包括直接和间接土地利用变化的影响,其生命周期排放比六种受管制的空气污染物的传统化石燃料大得多。排放量的大小和不确定性随着生命周期整合周期的延长而减小。结果取决于这里使用的单一 LUC 情景。在 LUC 不确定性之后,LUC 排放不确定性的最大来源来自森林砍伐期间的燃烧完全度。虽然巴西目前的生物燃料耕地燃烧政策旨在减少生命周期排放,但这些政策并没有解决间接土地利用变化造成的大量排放。