Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, United States.
Nano Lett. 2012 Sep 12;12(9):4590-4. doi: 10.1021/nl301844z. Epub 2012 Sep 4.
A two-dimensional (2D) electron gas system in an oxide heterostructure serves as an important playground for novel phenomena. Here, we show that, by using fractional δ-doping to control the interface's composition in La(x)Sr(1-x)TiO(3)/SrTiO(3) artificial oxide superlattices, the filling-controlled 2D insulator-metal transition can be realized. The atomic-scale control of d-electron band filling, which in turn contributes to the tuning of effective mass and density of the charge carriers, is found to be a fascinating route to substantially enhanced carrier mobilities.
二维(2D)电子气系统在氧化物异质结构中是一个重要的研究平台,可以用于探索新现象。在这里,我们展示了通过分数 δ 掺杂来控制 La(x)Sr(1-x)TiO(3)/SrTiO(3)人工氧化物超晶格界面的组成,可以实现填充控制的 2D 绝缘-金属转变。我们发现,通过对 d 电子能带填充的原子级控制,从而调节载流子的有效质量和密度,是提高载流子迁移率的一种很有前途的方法。