Department of Chemistry and Biochemistry, The University of Arizona, Tucson, AZ 85721, United States.
J Mass Spectrom. 2012 Oct;47(10):1364-71. doi: 10.1002/jms.3063.
It has been demonstrated that argininolysis and uricolysis are involved in the synthesis and excretion of urea in Aedes aegypti female mosquitoes. To further investigate the metabolic regulation of urea in female mosquitoes, it is desirable to have a rapid and efficient method to monitor arginine (Arg) concentration in mosquito excreta. Thus, a procedure currently used for the identification of Arg in urea cycle disorders in newborn babies was adapted to analyze Arg in A. aegypti excreta. The fragmentation patterns of the isobutyl esters of Arg and (15)N(2)-Arg (labeled at the guanidino group) were explored by electrospray ionization (ESI)-tandem mass spectrometry and fragmentation pathways not described before were characterized. In addition, Arg, (18)O(2)-Arg, (15)N(2)-Arg and (15)N(2)-(18)O(2)-Arg were also analyzed to elucidate some of the minor fragments in greater detail. Mosquito excreta from individual females were collected before and at different times after feeding a blood meal, mixed with (15)N(2)-Arg, an internal standard, and then derivatized as isobutyl esters. Based on the fragmentation mechanisms of Arg standards, studied by MS(2) and MS(3), Arg in the mosquito excreta was successfully analyzed by ESI-multiple reaction monitoring in a triple-quadrupole mass spectrometer. Arg excretion was monitored over a 120 h window before and after feeding female mosquitoes with a blood meal, with the maximum level of Arg excretion observed at 36-48 h post blood feeding. This method provides an efficient and rapid tool to quantify Arg in individual blood-fed mosquitoes, and can be applied to other organisms, whose small size severally limits the use of conventional biochemical analysis.
已经证明,精氨酸分解和尿酸分解参与了埃及伊蚊雌性蚊子中尿素的合成和排泄。为了进一步研究雌性蚊子中尿素的代谢调节,理想情况下需要有一种快速有效的方法来监测蚊子排泄物中的精氨酸 (Arg) 浓度。因此,适应了目前用于新生儿尿素循环障碍鉴定的程序,以分析埃及伊蚊排泄物中的 Arg。通过电喷雾电离 (ESI)-串联质谱探索了 Arg 和 (15)N(2)-Arg(胍基基团标记)的异丁基酯的碎裂模式,并描述了以前未描述的碎裂途径。此外,还分析了 Arg、(18)O(2)-Arg、(15)N(2)-Arg 和 (15)N(2)-(18)O(2)-Arg,以更详细地阐明一些次要片段。在喂食血餐后的不同时间,从单个雌性蚊子收集排泄物,与内部标准 (15)N(2)-Arg 混合,然后衍生为异丁基酯。基于 Arg 标准的 MS(2)和 MS(3) 研究的碎裂机制,通过 ESI-多重反应监测在三重四极杆质谱仪中成功分析了蚊子排泄物中的 Arg。在喂食血餐后的 120 小时窗口中监测 Arg 的排泄,在血液喂养后 36-48 小时观察到 Arg 排泄的最大值。该方法提供了一种有效且快速的工具来定量个体血食蚊子中的 Arg,并且可以应用于其他生物体,其小尺寸严重限制了常规生化分析的使用。