Department of Electrical and Computer Engineering, Rice University, Houston, Texas 77005, USA.
Nano Lett. 2012 Nov 14;12(11):6000-4. doi: 10.1021/nl303517v. Epub 2012 Oct 22.
The use of aluminum for plasmonic nanostructures opens up new possibilities, such as access to short-wavelength regions of the spectrum, complementary metal-oxide-semiconductor (CMOS) compatibility, and the possibility of low-cost, sustainable, mass-producible plasmonic materials. Here we examine the properties of individual Al nanorod antennas with cathodoluminescence (CL). This approach allows us to image the local density of optical states (LDOS) of Al nanorod antennas with a spatial resolution less than 20 nm and to identify the radiative modes of these nanostructures across the visible and into the UV spectral range. The results, which agree well with finite difference time domain (FDTD) simulations, lay the groundwork for precise Al plasmonic nanostructure design for a variety of applications.
铝在等离子体纳米结构中的应用开辟了新的可能性,例如可以进入光谱的短波长区域、与互补金属氧化物半导体(CMOS)兼容,以及实现低成本、可持续、大规模生产的等离子体材料。在这里,我们通过阴极发光(CL)研究了单个铝纳米棒天线的性质。这种方法使我们能够以小于 20nm 的空间分辨率对铝纳米棒天线的局域光密度状态(LDOS)进行成像,并在可见光谱到紫外光谱范围内识别这些纳米结构的辐射模式。这些结果与有限差分时域(FDTD)模拟吻合较好,为各种应用的精确铝等离子体纳米结构设计奠定了基础。