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掺杂单壁碳纳米管中激子-电子散射的抑制。

Suppression of exciton-electron scattering in doped single-walled carbon nanotubes.

机构信息

Graduate School of Pure and Applied Sciences, University of Tsukuba, Tsukuba, Ibaraki 305-8571, Japan.

出版信息

Phys Rev Lett. 2012 Nov 2;109(18):187403. doi: 10.1103/PhysRevLett.109.187403. Epub 2012 Oct 31.

Abstract

We theoretically study the phase relaxation of excitons in doped single-walled carbon nanotubes caused by elastic scattering between an exciton and an electron. Our calculation of the spectral linewidth, that is the inverse of the scattering rate, demonstrates that this dephasing process is unexpectedly suppressed in doped single-walled carbon nanotubes, giving rise to anomalous nonlinear behavior as a function of the electron density. A detailed investigation reveals that the logarithmic correction of the exciton self-energy plays a critical role in the exciton-carrier scattering dynamics.

摘要

我们从理论上研究了激子和电子之间的弹性散射引起的掺杂单壁碳纳米管中激子的相位弛豫。我们对线宽(散射率的倒数)的计算表明,掺杂单壁碳纳米管中的退相过程出人意料地受到抑制,从而导致反常的非线性行为,这与电子密度有关。详细的研究表明,激子自能的对数修正在激子-载流子散射动力学中起着关键作用。

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