Department of Chemistry, Center for Photochemical Sciences, Bowling Green State University, Bowling Green, Ohio 43403, United States.
Langmuir. 2013 Jan 22;29(3):950-6. doi: 10.1021/la303779y. Epub 2013 Jan 9.
We investigate the single-cell reduction of toxic Cr(VI) by the dissimilatory metal-reducing bacterium Shewanella oneidensis MR-1 (MR-1), an important bioremediation process, using Raman spectroscopy and scanning electron microscopy (SEM) combined with energy-dispersive X-ray spectroscopy (EDX). Our experiments indicate that the toxic, highly soluble Cr(VI) can be efficiently reduced to less toxic, nonsoluble Cr(2)O(3) nanoparticles by MR-1. Cr(2)O(3) is observed to emerge as nanoparticles adsorbed on the cell surface and its chemical nature is identified by EDX imaging and Raman spectroscopy. Co-localization of Cr(2)O(3) and cytochromes by EDX imaging and Raman spectroscopy suggests a terminal reductase role for MR-1 surface-exposed cytochromes MtrC and OmcA. Our experiments revealed that the cooperation of surface proteins OmcA and MtrC makes the reduction reaction most efficient, and the sequence of the reducing reactivity of MR-1 is wild type > single mutant ΔmtrC or mutant ΔomcA > double mutant (ΔomcA-ΔmtrC). Moreover, our results also suggest that direct microbial Cr(VI) reduction and Fe(II) (hematite)-mediated Cr(VI) reduction mechanisms may coexist in the reduction processes.
我们使用拉曼光谱和扫描电子显微镜(SEM)结合能量色散 X 射线光谱(EDX)研究了异化金属还原菌 Shewanella oneidensis MR-1(MR-1)将有毒 Cr(VI)还原为单细胞的过程,这是一种重要的生物修复过程。我们的实验表明,有毒的、高可溶性的 Cr(VI)可以被 MR-1 高效还原为毒性较低的、不溶性的 Cr2O3 纳米颗粒。通过 EDX 成像和拉曼光谱观察到 Cr2O3 以吸附在细胞表面的纳米颗粒形式出现,其化学性质通过 EDX 成像和拉曼光谱确定。EDX 成像和拉曼光谱显示 Cr2O3 和细胞色素的共定位表明 MR-1 表面暴露的细胞色素 MtrC 和 OmcA 具有末端还原酶的作用。我们的实验表明,表面蛋白 OmcA 和 MtrC 的合作使还原反应效率最高,MR-1 的还原反应活性顺序为野生型>单突变体ΔmtrC 或突变体ΔomcA>双突变体(ΔomcA-ΔmtrC)。此外,我们的结果还表明,直接微生物 Cr(VI)还原和 Fe(II)(赤铁矿)介导的 Cr(VI)还原机制可能在还原过程中同时存在。