Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA.
Phys Rev Lett. 2013 Jan 18;110(3):037003. doi: 10.1103/PhysRevLett.110.037003.
The nature of metallicity and the level of electronic correlations in the antiferromagnetically ordered parent compounds are two important open issues for the iron-based superconductivity. We perform a temperature-dependent angle-resolved photoemission spectroscopy study of Fe(1.02)Te, the parent compound for iron chalcogenide superconductors. Deep in the antiferromagnetic state, the spectra exhibit a "peak-dip-hump" line shape associated with two clearly separate branches of dispersion, characteristics of polarons seen in manganites and lightly doped cuprates. As temperature increases towards the Néel temperature (T(N)), we observe a decreasing renormalization of the peak dispersion and a counterintuitive sharpening of the hump linewidth, suggestive of an intimate connection between the weakening electron-phonon (e-ph) coupling and antiferromagnetism. Our finding points to the highly correlated nature of the Fe(1.02)Te ground state featured by strong interactions among the charge, spin, and lattice and a good metallicity plausibly contributed by the coherent polaron motion.
金属性的本质和反铁磁有序母体化合物中的电子关联程度是铁基超导电性的两个重要待解决问题。我们对铁硫族化合物超导体的母体化合物 Fe(1.02)Te 进行了依赖温度的角分辨光电子能谱研究。在反铁磁状态深处,光谱呈现出与两个明显分离的色散分支相关的“峰-谷-峰”线形状,这是锰氧化物和轻掺杂铜氧化物中极化子的特征。随着温度升高接近奈尔温度(T(N)),我们观察到峰色散的重整化减小,以及令人惊讶的峰线宽变尖锐,这表明电子-声子(e-ph)耦合和反铁磁有序之间存在密切联系。我们的发现指出了 Fe(1.02)Te 基态的强关联性质,其特点是电荷、自旋和晶格之间存在强烈相互作用,以及相干极化子运动可能导致的良好金属性。