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近藤相互作用在 FeTe 中的表现及其在磁性有序中的潜在作用。

Kondo interaction in FeTe and its potential role in the magnetic order.

机构信息

Center for Correlated Electron Systems, Institute for Basic Science, Seoul, 08826, Korea.

Department of Physics & Astronomy, Seoul National University, Seoul, 08826, Korea.

出版信息

Nat Commun. 2023 Jul 12;14(1):4145. doi: 10.1038/s41467-023-39827-1.

Abstract

Finding d-electron heavy fermion states has been an important topic as the diversity in d-electron materials can lead to many exotic Kondo effect-related phenomena or new states of matter such as correlation-driven topological Kondo insulator. Yet, obtaining direct spectroscopic evidence for a d-electron heavy fermion system has been elusive to date. Here, we report the observation of Kondo lattice behavior in an antiferromagnetic metal, FeTe, via angle-resolved photoemission spectroscopy, scanning tunneling spectroscopy and transport property measurements. The Kondo lattice behavior is represented by the emergence of a sharp quasiparticle and Fano-type tunneling spectra at low temperatures. The transport property measurements confirm the low-temperature Fermi liquid behavior and reveal successive coherent-incoherent crossover upon increasing temperature. We interpret the Kondo lattice behavior as a result of hybridization between localized Fe 3d and itinerant Te 5p orbitals. Our observations strongly suggest unusual cooperation between Kondo lattice behavior and long-range magnetic order.

摘要

发现 d 电子重费米子态一直是一个重要的研究课题,因为 d 电子材料的多样性可以导致许多奇特的与 Kondo 效应相关的现象或物质的新态,如关联驱动的拓扑 Kondo 绝缘体。然而,到目前为止,获得 d 电子重费米子体系的直接光谱证据一直难以实现。在这里,我们通过角分辨光发射谱、扫描隧道谱和输运性质测量,报告了在反铁磁金属 FeTe 中观察到的 Kondo 晶格行为。低温下出现尖锐的准粒子和 Fano 型隧道谱,代表了 Kondo 晶格行为。输运性质测量证实了低温费米液体行为,并揭示了随着温度升高的连续相干-非相干交叉。我们将 Kondo 晶格行为解释为局域 Fe 3d 和巡游 Te 5p 轨道之间的杂化作用的结果。我们的观察强烈表明 Kondo 晶格行为与长程磁有序之间存在不寻常的合作。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2225/10338437/015c72caf6e5/41467_2023_39827_Fig1_HTML.jpg

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