Center for Correlated Electron Systems, Institute for Basic Science, Seoul, 08826, Korea.
Department of Physics & Astronomy, Seoul National University, Seoul, 08826, Korea.
Nat Commun. 2023 Jul 12;14(1):4145. doi: 10.1038/s41467-023-39827-1.
Finding d-electron heavy fermion states has been an important topic as the diversity in d-electron materials can lead to many exotic Kondo effect-related phenomena or new states of matter such as correlation-driven topological Kondo insulator. Yet, obtaining direct spectroscopic evidence for a d-electron heavy fermion system has been elusive to date. Here, we report the observation of Kondo lattice behavior in an antiferromagnetic metal, FeTe, via angle-resolved photoemission spectroscopy, scanning tunneling spectroscopy and transport property measurements. The Kondo lattice behavior is represented by the emergence of a sharp quasiparticle and Fano-type tunneling spectra at low temperatures. The transport property measurements confirm the low-temperature Fermi liquid behavior and reveal successive coherent-incoherent crossover upon increasing temperature. We interpret the Kondo lattice behavior as a result of hybridization between localized Fe 3d and itinerant Te 5p orbitals. Our observations strongly suggest unusual cooperation between Kondo lattice behavior and long-range magnetic order.
发现 d 电子重费米子态一直是一个重要的研究课题,因为 d 电子材料的多样性可以导致许多奇特的与 Kondo 效应相关的现象或物质的新态,如关联驱动的拓扑 Kondo 绝缘体。然而,到目前为止,获得 d 电子重费米子体系的直接光谱证据一直难以实现。在这里,我们通过角分辨光发射谱、扫描隧道谱和输运性质测量,报告了在反铁磁金属 FeTe 中观察到的 Kondo 晶格行为。低温下出现尖锐的准粒子和 Fano 型隧道谱,代表了 Kondo 晶格行为。输运性质测量证实了低温费米液体行为,并揭示了随着温度升高的连续相干-非相干交叉。我们将 Kondo 晶格行为解释为局域 Fe 3d 和巡游 Te 5p 轨道之间的杂化作用的结果。我们的观察强烈表明 Kondo 晶格行为与长程磁有序之间存在不寻常的合作。