Department of Chemistry and Center for Theoretical Studies, Indian Institute of Technology Kharagpur, India.
Chemphyschem. 2013 Aug 5;14(11):2511-7. doi: 10.1002/cphc.201300357. Epub 2013 Jun 3.
The noble gas binding ability of CN3Be3(+) clusters was assessed both by ab intio and density functional studies. The global minimum structure of the CN3Be3(+) cluster binds with four noble-gas (NG) atoms, in which the Be atoms are acting as active centers. The electron transfer from the noble gas to the Be atom plays a key role in binding. The dissociation energy of the Be-NG bond gradually increases from He to Rn, maintaining the periodic trend. The HOMO-LUMO gap, an indicator for stability, gives additional insight into these NG-bound clusters. The temperature at which the NG-binding process is thermodynamically feasible was identified. In addition, we investigated the stability of two new neutral NG compounds, (NG)BeSe and (NG)BeTe, and found them to be suitable candidates to be detected experimentally such as (NG)BeO and (NG)BeS. The dissociation energies of the Be-NG bond in monocationic analogues of (NG)BeY (Y=O, S, Se, Te) were found to be larger than in the corresponding neutral counter-parts. Finally, the higher the positive charge on the Be atoms, the higher the dissociation energy for the Be-NG bond becomes.
采用从头算和密度泛函研究方法评估了 CN3Be3(+) 团簇对稀有气体的结合能力。CN3Be3(+) 团簇的全局最小结构结合了四个稀有气体 (NG) 原子,其中 Be 原子充当活性中心。稀有气体向 Be 原子的电子转移在结合中起着关键作用。Be-NG 键的离解能从 He 到 Rn 逐渐增加,保持了周期性趋势。HOMO-LUMO 能隙是稳定性的一个指标,为这些 NG 结合团簇提供了额外的见解。确定了 NG 结合过程在热力学上可行的温度。此外,我们还研究了两种新的中性 NG 化合物 (NG)BeSe 和 (NG)BeTe 的稳定性,并发现它们是适合实验检测的候选物,如 (NG)BeO 和 (NG)BeS。在 (NG)BeY(Y=O、S、Se、Te)的一价类似物中,Be-NG 键的离解能大于相应的中性对应物。最后,Be 原子上的正电荷越高,Be-NG 键的离解能就越高。