Akselrod Gleb M, Young Elizabeth R, Bradley M Scott, Bulović Vladimir
Organic and Nanostructured Electronics Laboratory, 77 Massachusetts Ave, Massachusetts Institute of Technology, Cambridge, MA 02139, USA.
Opt Express. 2013 May 20;21(10):12122-8. doi: 10.1364/OE.21.012122.
We demonstrate room temperature lasing through the polaritonic mode of a J-aggregate microcavity in which losses from exciton-exciton annihilation and slow polariton relaxation typical of direct J-aggregate excitation are circumvented via intra-cavity pumping. The pumping scheme utilizes an organic dye layer (DCM) within the cavity with an emission band overlapping the entire lower J-aggregate polariton branch spectrum, hence forcing DCM lasing to occur through the strongly-coupled mode. This cavity architecture, which separates strong coupling and gain into two materials, presents a general and flexible design for polariton devices and allows for the use of a wide range of materials, organic and inorganic, to be integrated into the cavity.
我们通过J聚集体微腔的极化激元模式展示了室温激光发射,其中通过腔内泵浦规避了激子-激子湮灭以及直接J聚集体激发典型的慢极化激元弛豫所带来的损耗。该泵浦方案利用腔内的有机染料层(DCM),其发射带与整个较低的J聚集体极化激元分支光谱重叠,从而迫使DCM通过强耦合模式发生激光发射。这种将强耦合和增益分离到两种材料中的腔结构,为极化激元器件提供了一种通用且灵活的设计,并允许将多种有机和无机材料集成到腔内。