Dipartimento di Fisica e Scienze della Terra, Università di Ferrara, I-44122 Ferrara, Italy.
J Phys Condens Matter. 2013 Sep 25;25(38):386001. doi: 10.1088/0953-8984/25/38/386001. Epub 2013 Aug 29.
The magnetothermal behavior of antiferromagnetic IrMn layers of different thickness (3, 6, 10 nm) has been studied by exploiting the exchange coupling with a ferromagnetic 5 nm-thick NiFe layer. A procedure has been devised for the measurement of the magnetization of the NiFe/IrMn bilayers as a function of temperature and time at different values of an external magnetic field, Hinv, antiparallel to the unidirectional exchange anisotropy. This analysis allows one to probe the effective distribution of anisotropy energy barriers of the antiferromagnetic phase, as sensed by the ferromagnetic layer. Two magnetic regimes have been distinguished. At temperature T < 100 K, the interfacial IrMn spins are frozen in a glassy state and are collectively involved in the exchange coupling with the NiFe spins. At T ∼ 100 K the collective state breaks up; thus, above this temperature, only the interfacial IrMn spins which are tightly polarized by the IrMn nanograins, forming the bulk of the layer, are effectively involved in the exchange coupling mechanism. Due to that, for T > 100 K the exchange coupling is ruled by the anisotropy energy barriers of the bulk IrMn nanograins, namely by the layer thickness. The thermal evolution of the exchange field and of the coercivity in the three samples is coherently explained in the framework of this description of the dynamic magnetic behavior of the IrMn phase.
不同厚度(3、6、10nm)的反铁磁 IrMn 层的磁热行为通过利用与铁磁 5nm 厚 NiFe 层的交换耦合来研究。设计了一种程序,用于在反铁磁各向异性的外磁场 Hinv 反平行于不同值的情况下,测量 NiFe/IrMn 双层的温度和时间的磁化强度。这种分析允许探测反铁磁相的各向异性能量势垒的有效分布,由铁磁层感知。已经区分了两种磁状态。在温度 T<100K 下,界面 IrMn 自旋被冻结在玻璃态中,并集体参与与 NiFe 自旋的交换耦合。在 T∼100K 时,集体状态会破裂;因此,高于此温度,只有由 IrMn 纳米颗粒紧密极化的界面 IrMn 自旋,形成层的大部分,才会有效地参与交换耦合机制。因此,对于 T>100K,交换耦合由体 IrMn 纳米颗粒的各向异性能量势垒决定,即由层厚度决定。在这种 IrMn 相动态磁行为描述的框架内,一致地解释了三个样品中交换场和矫顽力的热演化。