IV. Physical Institute, University of Göttingen, 37077 Göttingen, Germany.
Phys Rev Lett. 2013 Aug 23;111(8):085001. doi: 10.1103/PhysRevLett.111.085001. Epub 2013 Aug 20.
We present a study of the highly nonlinear optical excitation of noble gases in tapered hollow waveguides using few-femtosecond laser pulses. The local plasmonic field enhancement induces the generation of a nanometric plasma, resulting in incoherent extreme-ultraviolet fluorescence from optical transitions of neutral and ionized xenon, argon, and neon. Despite sufficient intensity in the waveguide, high-order harmonic generation is not observed. The fluorescent emission exhibits a strong bistability manifest as an intensity hysteresis, giving strong indications for multistep collisional excitations.
我们研究了使用飞秒激光脉冲在锥形中空波导中对稀有气体的高度非线性光学激发。局部等离子体场增强诱导纳米级等离子体的产生,从而导致中性和离子态氙气、氩气和氖气的光学跃迁产生非相干极紫外荧光。尽管在波导中有足够的强度,但没有观察到高阶谐波产生。荧光发射表现出强烈的双稳性,表现为强度滞后,强烈表明存在多步碰撞激发。