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纳米等离子体近场阿秒脉冲的相位匹配。

Nano-plasmonic near field phase matching of attosecond pulses.

机构信息

LIDYL, CEA, CNRS, Université Paris-Saclay, CEA Saclay, 91191, Gif-sur-Yvette, France.

Leibniz Universität Hannover, Institut für Quantenoptik, Welfengarten 1, D-30167, Hannover, Germany.

出版信息

Sci Rep. 2017 Jul 25;7(1):6356. doi: 10.1038/s41598-017-06491-7.

Abstract

Nano-structures excited by light can enhance locally the electric field when tuned to plasmonic resonances. This phenomenon can be used to boost non-linear processes such as harmonic generation in crystals or in gases, Raman excitation, and four wave mixing. Here we present a theoretical investigation of the near-field phase matching of attosecond pulses emitted by high-order harmonic generation (HHG) of an atom immersed in a multi-cycle femtosecond infrared laser field and a spatially inhomogeneous plasmonic field. We demonstrate that the spatial inhomogeneity factor of the plasmonic field strongly affects the electron trajectory and recombination time which can be used to control the attosecond emission. For further insight into the plasmonic field effect, we monitor the phase of each quantum path as a function of the inhomogeneity strength. Moreover, we investigate the attosecond emission as a function of near-field phase matching effects. This is achieved by calculating the coherent field superposition of attosecond pulses emitted from various intensities or field inhomogeneities. Finally, far-field and near-field phase matching effects are combined to modulate the harmonic spectral phase towards the emission of a single attosecond pulse.

摘要

受光激发的纳米结构在调谐到等离子体共振时可以增强局部电场。这种现象可用于增强非线性过程,如晶体或气体中的谐波产生、拉曼激发和四波混频。在这里,我们对处于多周期飞秒红外激光场和空间非均匀等离子体场中的原子的高阶谐波产生(HHG)发射的阿秒脉冲的近场相位匹配进行了理论研究。我们证明了等离子体场的空间非均匀性因子强烈影响电子轨迹和复合时间,这可用于控制阿秒发射。为了更深入地了解等离子体场的影响,我们监测了每个量子路径的相位随不均匀性强度的变化。此外,我们还研究了阿秒发射作为近场相位匹配效应的函数。这是通过计算从不同强度或场不均匀性发出的阿秒脉冲的相干场叠加来实现的。最后,将远场和近场相位匹配效应相结合,以调制谐波光谱相位,从而发射单个阿秒脉冲。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/84a8/5527109/d23b42a9d9f5/41598_2017_6491_Fig1_HTML.jpg

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