CRISMAT, CNRS-ENSICAEN, Caen, France.
J Phys Condens Matter. 2013 Oct 16;25(41):416002. doi: 10.1088/0953-8984/25/41/416002. Epub 2013 Sep 11.
We performed magnetic and ferroelectric measurements, associated with Landau theory and symmetry analysis, in order to clarify the situation of the YMnO3 system, a classical example of type I multiferroics. We found that the only magnetic group compatible with all experimental data (neutron scattering, magnetization, polarization, dielectric constant, second harmonic generation) is the P6'(3) group. In this group a small ferromagnetic component along c is induced by the Dzyaloshinskii-Moriya interaction, and observed here in magnetization measurements. We found that the ferromagnetic and antiferromagnetic components can only be switched simultaneously, while the magnetic orders are functions of the polarization square and therefore insensitive to its sign.
我们进行了磁性和铁电测量,并结合朗道理论和对称分析,以澄清 YMnO3 系统的情况,这是一类 I 型多铁性的经典范例。我们发现,唯一与所有实验数据(中子散射、磁化、极化、介电常数、二次谐波产生)兼容的磁群是 P6'(3)群。在这个群中,由 Dzyaloshinskii-Moriya 相互作用诱导出一个沿 c 方向的小铁磁分量,我们在磁化测量中观察到了这一点。我们发现,铁磁和反铁磁分量只能同时切换,而磁序是极化平方的函数,因此对其符号不敏感。