The Blackett Laboratory, Department of Physics, Imperial College London, London SW7 2AZ, United Kingdom.
Phys Rev Lett. 2013 Aug 30;111(9):093901. doi: 10.1103/PhysRevLett.111.093901. Epub 2013 Aug 26.
Surface plasmons on metals can concentrate light into subnanometric volumes and on these near atomic length scales the electronic response at the metal interface is smeared out over a Thomas-Fermi screening length. This nonlocality is a barrier to a good understanding of atomic scale response to light and complicates the practical matter of computing the fields. In this Letter, we present a local analogue model and show that spatial nonlocality can be represented by replacing the nonlocal metal with a composite material, comprising a thin dielectric layer on top of a local metal. This method not only makes possible the quantitative analysis of nonlocal effects in complex plasmonic phenomena with unprecedented simplicity and physical insight, but also offers great practical advantages in their numerical treatment.
金属表面等离激元可以将光集中到亚纳米体积中,在这些近原子长度尺度上,金属界面的电子响应在托马斯-费米屏蔽长度上扩散开来。这种非局域性是对光的原子尺度响应进行良好理解的障碍,并使计算场的实际问题变得复杂。在这封信中,我们提出了一个局部模拟模型,并表明通过用复合材料替代非局部金属,即顶部有一层薄介电层的局部金属,可以表示空间非局域性。这种方法不仅可以以前所未有的简单性和物理洞察力对复杂等离子体现象中的非局域效应进行定量分析,而且在其数值处理方面也具有很大的实际优势。