Adriaens Annemie, Quinn Paul, Nikitenko Sergey, Dowsett Mark G
Department of Analytical Chemistry, Ghent University , Krijgslaan 281 S12, B9000, Ghent, Belgium.
Anal Chem. 2013 Oct 15;85(20):9556-63. doi: 10.1021/ac401646q. Epub 2013 Sep 30.
In experiments preliminary to the design of an X-ray-excited optical luminescence (XEOL)-based chemical mapping tool we have used X-ray micro (4.5 × 5.2 μm) and macro (1 × 6 mm) beams with similar total fluxes to assess the effects of a high flux density beam of X-rays at energies close to an absorption edge on inorganic surfaces in air. The near surface composition of corroded cupreous alloys was analyzed using parallel X-ray and optical photoemission channels to collect X-ray absorption near-edge structure (XANES) data at the Cu K edge. The X-ray fluorescence channel is characteristic of the composition averages over several micrometers into the surface, whereas the optical channel is surface specific to about 200 nm. While the X-ray fluorescence data were mostly insensitive to the X-ray dose, the XEOL-XANES data from the microbeam showed significant dose-dependent changes to the superficial region, including surface cleaning, changes in the oxidation state of the copper, and destruction of surface compounds responsible for pre-edge fluorescence or phosphorescence in the visible. In one case, there was evidence that the lead phase in a bronze had melted. Conversely, data from the macrobeam were stable over several hours. Apart from localized heating effects, the microbeam damage is probably associated with the O3 loading of the surface and increased reaction rate with atmospheric water vapor.
在设计基于X射线激发光致发光(XEOL)的化学绘图工具的前期实验中,我们使用了具有相似总通量的X射线微束(4.5×5.2μm)和宏束(1×6mm),以评估能量接近吸收边的高通量密度X射线束对空气中无机表面的影响。使用平行的X射线和光发射通道分析腐蚀的铜合金的近表面成分,以收集Cu K边的X射线吸收近边结构(XANES)数据。X射线荧光通道表征的是表面以下几微米范围内的成分平均值,而光通道则对约200nm的表面具有特异性。虽然X射线荧光数据大多对X射线剂量不敏感,但来自微束的XEOL-XANES数据显示,表面区域存在明显的剂量依赖性变化,包括表面清洁、铜氧化态的变化以及导致可见光中前缘荧光或磷光的表面化合物的破坏。在一个案例中,有证据表明青铜中的铅相已经熔化。相反,来自宏束的数据在几个小时内是稳定的。除了局部加热效应外,微束损伤可能与表面的O3负载以及与大气水蒸气的反应速率增加有关。