Department of Physics and Astronomy, University of North Carolina , Chapel Hill, North Carolina 27599-3255, United States.
J Phys Chem B. 2013 Oct 10;117(40):12007-12. doi: 10.1021/jp407115j. Epub 2013 Oct 2.
Numerous small molecules exhibit drug-like properties by low-affinity binding to proteins. Such binding is known to be influenced by water, the detailed picture of which, however, remains unclear. One particular example is the controversial role of water in the binding of general anesthetics to proteins as an essential step in general anesthesia. Here we demonstrate that a critical amount of hydration water is a prerequisite for anesthetic-protein binding. Using nuclear magnetic resonance, the concurrent adsorption of hydration water and bound anesthetics on model proteins are simultaneously measured. Halothane binding on proteins can only take place after protein hydration reaches a threshold hydration level of ∼0.31 g of water/g of proteins at the relative water vapor pressure of ∼0.95. Similar dependence on hydration is also observed for several other anesthetics. The ratio of anesthetic partial pressures at which two different anesthetics reach the same fractional load is correlated with the anesthetic potency. The binding of nonimmobilizers, which are structurally similar to known anesthetics but unable to produce anesthesia, does not occur even after the proteins are fully hydrated. Our results provide the first unambiguous experimental evidence that water is absolutely required to enable anesthetic-protein interactions, shedding new light on the general mechanism of molecular recognition and binding.
许多小分子通过与蛋白质的低亲和力结合表现出药物样特性。这种结合被认为受到水的影响,然而,水的详细情况仍不清楚。一个特别的例子是水在全身麻醉中作为蛋白质与全身麻醉剂结合的关键步骤中的争议作用。在这里,我们证明了一定量的水合作用是麻醉蛋白结合的先决条件。我们使用核磁共振技术,同时测量模型蛋白质上结合水和结合麻醉剂的协同吸附。只有在蛋白质水合作用达到相对水蒸气压力约为 0.95 时约 0.31 g 水/g 蛋白质的阈值水合水平后,卤烷才能在蛋白质上结合。其他几种麻醉剂也观察到类似的水合依赖性。两种不同麻醉剂达到相同分数负荷时的麻醉剂分压比与麻醉剂效力相关。即使蛋白质完全水合,非固定剂(其结构与已知麻醉剂相似但不能产生麻醉)的结合也不会发生。我们的结果提供了第一个明确的实验证据,证明水是使麻醉蛋白相互作用绝对必需的,为分子识别和结合的一般机制提供了新的认识。