Virginia Polytechnic Institute and State University , Blacksburg, Virginia 24061, United States.
Environ Sci Technol. 2014;48(1):747-52. doi: 10.1021/es403363v. Epub 2013 Dec 20.
Mercury (Hg) dynamics in the Arctic is receiving increasing attention, but further understanding is limited by a lack of studies in Russia, which encompasses the majority of the pan-Arctic watershed. This study reports Hg concentrations and trends in burbot (Lota lota) from the Lena and Mezen Rivers in the Russian Arctic, and assesses the extent to which they differ from those found in burbot in arctic rivers elsewhere. Mercury concentrations in burbot in the Lena and Mezen Rivers were found to be generally lower than in 23 other locations, most of which are in the Mackenzie River Basin (Canada). Mercury concentrations in burbot in the Lena and Mezen Rivers also were found to have been declining at an annual rate of 2.3% while they have been increasing in the Mackenzie River Basin at annual rates between 2.2 and 5.1% during roughly the same time period. These contrasting patterns in Hg in burbot across the pan-Arctic may be explained by geographic heterogeneity in controlling processes, including riverine particulate material loads, historically changing atmospheric inputs, postdepositional processes, and climate change impacts.
汞(Hg)在北极的动态变化正受到越来越多的关注,但由于俄罗斯缺乏相关研究,对其的了解仍然有限,而俄罗斯涵盖了泛北极流域的大部分地区。本研究报告了来自俄罗斯北极地区勒拿河和梅曾河的欧白鲑(Lota lota)体内的汞浓度和变化趋势,并评估了它们与其他北极地区河流中的欧白鲑体内汞浓度的差异程度。研究发现,勒拿河和梅曾河中的欧白鲑体内的汞浓度普遍低于其他 23 个地点,其中大部分位于麦肯齐河流域(加拿大)。研究还发现,勒拿河和梅曾河中的欧白鲑体内的汞浓度呈每年 2.3%的下降趋势,而在同一时期,麦肯齐河流域的汞浓度呈每年 2.2%至 5.1%的上升趋势。在整个泛北极地区,欧白鲑体内汞的这种对比模式可以用控制过程中的地理异质性来解释,包括河流颗粒物质负荷、历史上不断变化的大气输入、沉积后过程和气候变化影响。