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原子层沉积法制备可转移 Al(2)O(3)纳米片用于石墨烯 FET

Fabrication of transferable Al(2)O(3) nanosheet by atomic layer deposition for graphene FET.

机构信息

Nanodevice Laboratory, School of Electrical and Electronic Engineering, and §Nanobio Device Laboratory, School of Electrical and Electronic Engineering, Yonsei University , Seodaemun-Gu, Seoul 120-749, Republic of Korea.

出版信息

ACS Appl Mater Interfaces. 2014 Feb 26;6(4):2764-9. doi: 10.1021/am4052987. Epub 2014 Feb 11.

Abstract

Without introducing defects in the monolayer of carbon lattice, the deposition of high-κ dielectric material is a significant challenge because of the difficulty of high-quality oxide nucleation on graphene. Previous investigations of the deposition of high-κ dielectrics on graphene have often reported significant degradation of the electrical properties of graphene. In this study, we report a new way to integrate high-κ dielectrics with graphene by transferring a high-κ dielectric nanosheet onto graphene. Al2O3 film was deposited on a sacrificial layer using an atomic layer deposition process and the Al2O3 nanosheet was fabricated by removing the sacrificial layer. Top-gated graphene field-effect transistors were fabricated and characterized using the Al2O3 nanosheet as a gate dielectric. The top-gated graphene was demonstrated to have a field-effect mobility up to 2200 cm(2)/(V s). This method provides a new method for high-performance graphene devices with broad potential impacts reaching from high-frequency high-speed circuits to flexible electronics.

摘要

在不引入碳原子层单层缺陷的情况下,由于在石墨烯上高质量氧化物成核的困难,高κ介电材料的沉积是一个重大挑战。先前关于在石墨烯上沉积高κ电介质的研究经常报告石墨烯的电性能显著下降。在这项研究中,我们报告了一种通过将高κ介电纳米片转移到石墨烯上来与石墨烯集成高κ介电材料的新方法。使用原子层沉积工艺在牺牲层上沉积 Al2O3 薄膜,并通过去除牺牲层来制造 Al2O3 纳米片。使用 Al2O3 纳米片作为栅介质制造顶栅石墨烯场效应晶体管并对其进行了表征。所制造的顶栅石墨烯表现出高达 2200 cm2/(V s)的场效应迁移率。这种方法为高性能石墨烯器件提供了一种新方法,其潜在影响广泛,从高频高速电路到柔性电子学。

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