Makhotkin Igor A, Zoethout Erwin, van de Kruijs Robbert, Yakunin Sergey N, Louis Eric, Yakunin A M, Banine V, Müllender S, Bijkerk Fred
Opt Express. 2013 Dec 2;21(24):29894-904. doi: 10.1364/OE.21.029894.
In the first part of this article we experimentally show that contrast between the very thin layers of La and B enables close to theoretical reflectance. The reflectivity at 6.8 nm wavelength was measured from La/B multilayer mirrors with period thicknesses ranging from 3.5 to 7.2 nm at the appropriate angle for constructive interference. The difference between the measured reflectance and the reflectance calculated for a perfect multilayer structure decreases with increasing multilayer period. The reflectance of the multilayer with the largest period approaches the theoretical value, showing that the optical contrast between the very thin layers of these structures allows to experimentally access close to theoretical reflectance. In the second part of the article we discuss the structure of La/B and LaN/B multilayers. This set of multilayers is probed by hard X-rays (λ = 0.154 nm) and EUV radiation (λ = 6.8 nm). The structure is reconstructed based on a simultaneous fit of the grazing incidence hard X-ray reflectivity and the EUV reflectivity curves. The reflectivity analysis of the La/B and LaN/B multilayer mirrors shows that the lower reflectance of La/B mirrors compared to LaN/B mirrors can be explained by the presence of 5% of La atoms in the B layer and 63% of B in La layer. After multi-parametrical optimization of the LaN/B system, including the nitridation of La, the highest near normal incidence reflectivity of 57.3% at 6.6 nm wavelength has been measured from a multilayer mirror, containing 175 bi-layers. This is the highest value reported so far.
在本文的第一部分,我们通过实验表明,镧(La)和硼(B)的超薄层之间的对比度能够实现接近理论值的反射率。在6.8纳米波长下,从周期厚度在3.5至7.2纳米范围内的La/B多层镜中,以产生相长干涉的合适角度测量反射率。随着多层周期的增加,测量的反射率与为完美多层结构计算的反射率之间的差异减小。具有最大周期的多层镜的反射率接近理论值,表明这些结构的超薄层之间的光学对比度使得能够通过实验获得接近理论的反射率。在本文的第二部分,我们讨论了La/B和LaN/B多层膜的结构。这组多层膜通过硬X射线(波长λ = 0.154纳米)和极紫外辐射(波长λ = 6.8纳米)进行探测。基于掠入射硬X射线反射率和极紫外反射率曲线的同时拟合来重建结构。对La/B和LaN/B多层镜的反射率分析表明,与LaN/B镜相比,La/B镜较低的反射率可归因于B层中存在5%的La原子以及La层中存在63%的B原子。在对LaN/B系统进行多参数优化(包括La的氮化)之后,从包含175个双层的多层镜中,在6.6纳米波长处测量到了高达57.3%的近正入射反射率。这是迄今为止报道的最高值。