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从饮用水基础设施中清除放射性药剂:文献综述与总结。

Decontamination of radiological agents from drinking water infrastructure: a literature review and summary.

机构信息

United States Environmental Protection Agency, National Homeland Security Research Center (NG-16), 26 W. Martin Luther King Dr., Cincinnati, OH 45268, United States.

United States Environmental Protection Agency, National Homeland Security Research Center (NG-16), 26 W. Martin Luther King Dr., Cincinnati, OH 45268, United States.

出版信息

Environ Int. 2014 Nov;72:129-32. doi: 10.1016/j.envint.2014.01.020. Epub 2014 Feb 13.

DOI:10.1016/j.envint.2014.01.020
PMID:24529629
Abstract

This report summarizes the current state of knowledge on the persistence of radiological agents on drinking water infrastructure (such as pipes) along with information on decontamination should persistence occur. Decontamination options for drinking water infrastructure have been explored for some important radiological agents (cesium, strontium and cobalt), but important data gaps remain. Although some targeted experiments have been published on cesium, strontium and cobalt persistence on drinking water infrastructure, most of the data comes from nuclear clean-up sites. Furthermore, the studies focused on drinking water systems use non-radioactive surrogates. Non-radioactive cobalt was shown to be persistent on iron due to oxidation with free chlorine in drinking water and precipitation on the iron surface. Decontamination with acidification was an effective removal method. Strontium persistence on iron was transient in tap water, but adherence to cement-mortar has been demonstrated and should be further explored. Cesium persistence on iron water infrastructure was observed when flow was stagnant, but not with water flow present. Future research suggestions focus on expanding the available cesium, strontium and cobalt persistence data to other common infrastructure materials, specifically cement-mortar. Further exploration chelating agents and low pH treatment is recommended for future decontamination studies.

摘要

本报告总结了放射性物质在饮用水基础设施(如管道)上持续存在的现有知识状况,并提供了持续存在时的去污信息。已经针对一些重要的放射性物质(铯、锶和钴)探索了饮用水基础设施的去污选择,但仍存在重要的数据空白。尽管已经发表了一些关于铯、锶和钴在饮用水基础设施上持续存在的针对性实验,但大部分数据来自核清理现场。此外,这些研究侧重于使用非放射性示踪剂的饮用水系统。非放射性钴由于在饮用水中与游离氯发生氧化以及在铁表面沉淀而在铁上持续存在。酸化的去污是一种有效的去除方法。锶在自来水中对铁的持续存在是短暂的,但已经证明了对水泥-砂浆的附着,应该进一步探索。当水流停滞时,铯在铁制水基础设施上持续存在,但当水流存在时则不存在。未来的研究建议侧重于将现有的铯、锶和钴持续存在数据扩展到其他常见的基础设施材料,特别是水泥-砂浆。建议进一步探索螯合剂和低 pH 值处理,作为未来去污研究的选择。

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