European Synchrotron Radiation Facility, 38043, Grenoble, France.
Adv Mater. 2014 Dec 10;26(46):7873-9. doi: 10.1002/adma.201304345. Epub 2014 Mar 27.
Semiconductor nanowires offer new opportunities for optoelectronic and spintronic nanodevices. However, their full potential is ultimately dictated by our ability to control multiple property-function relationships taking place at the nanoscale in the spatial and time domains. Only a combination of high-resolution analytical techniques can provide a comprehensive understanding of their complex functionalities. Here we describe how a multimodal hard X-ray nanoprobe addresses fundamental questions in nanowire research. Selected topics ranging from cluster formation, dopant segregation, and phase separations to quantum confinement effects are investigated with sub-100 nm spatial resolution and sub-50 ps temporal resolution. This approach opens new avenues for structural, composition and optical studies with broad applicability in materials science.
半导体纳米线为光电和自旋电子纳米器件提供了新的机会。然而,它们的全部潜力最终取决于我们控制纳米尺度上在空间和时间域中发生的多个性能-功能关系的能力。只有结合高分辨率分析技术才能全面了解它们复杂的功能。在这里,我们描述了一种多模式硬 X 射线纳米探针如何解决纳米线研究中的基本问题。选择的主题范围从团簇形成、掺杂剂偏析和相分离到量子限制效应,都具有亚 100nm 的空间分辨率和亚 50ps 的时间分辨率。这种方法为结构、成分和光学研究开辟了新的途径,在材料科学中有广泛的应用。