Rubbiani Riccardo, Salassa Luca, de Almeida Andreia, Casini Angela, Ott Ingo
Institute of Medicinal and Pharmaceutical Chemistry, Technische Universität Braunschweig, Beethovenstrasse 55, 38106 Braunschweig (Germany).
ChemMedChem. 2014 Jun;9(6):1205-10. doi: 10.1002/cmdc.201400056. Epub 2014 Mar 26.
Organometallic gold complexes with N-heterocyclic carbene (NHC) ligands have been demonstrating promising properties as novel anticancer agents. Gold(I) NHC complexes containing different phosphanes as secondary ligands were shown to trigger strong cytotoxic effects in cancer cells, and their effective uptake into the cells was quantified by atomic absorption spectroscopy. Moreover, the new compounds strongly inhibited the activity of the seleno-enzyme thioredoxin reductase (TrxR) and of the zinc-finger enzyme poly(ADP-ribose) polymerase 1 (PARP-1). In the case of TrxR inhibition, their activity depended clearly on the size of the alkyl/aryl residues of phosphorus atoms. Density functional theory (DFT) calculations showed that the Au-P bond of the triphenylphosphane complex [Au(I) (NHC)(PPh3 )]I had a lower bond dissociation energy compared to trialkylphosphane complexes [Au(I) (NHC)(PR3 )]I, indicating a higher kinetic reactivity of this particular compound. In fact, [Au(I) (NHC)(PPh3 )]I triggered an enhanced inhibitory activity against PARP-1.
含有氮杂环卡宾(NHC)配体的有机金属金配合物已展现出作为新型抗癌剂的良好特性。含有不同膦作为二级配体的金(I)NHC配合物在癌细胞中表现出强烈的细胞毒性作用,并且通过原子吸收光谱法定量了它们在细胞中的有效摄取量。此外,这些新化合物强烈抑制了硒酶硫氧还蛋白还原酶(TrxR)和锌指酶聚(ADP - 核糖)聚合酶1(PARP - 1)的活性。在TrxR抑制的情况下,它们的活性明显取决于磷原子的烷基/芳基残基的大小。密度泛函理论(DFT)计算表明,与三烷基膦配合物[Au(I)(NHC)(PR3)]I相比,三苯基膦配合物[Au(I)(NHC)(PPh3)]I的Au - P键具有较低的键解离能,表明该特定化合物具有更高的动力学反应活性。事实上,[Au(I)(NHC)(PPh3)]I对PARP - 1引发了增强的抑制活性。